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云母/TiO2/Fe2O3复合材料
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY · 2020 · IF 3.306

A novel ternary Mica/TiO2/Fe2O3 composite pearlescent pigment for the photocatalytic degradation of acetaldehyde

Xiangming Fang,Guanhong Lu,Asad Mahmood,Zhihong Tang,Ziwei Liu,Linlin Zhang,Yan Wang,Jing Sun

A novel ternary mica/TiO 2 /Fe 2 O 3 composite pearlescent pigment has been designed for the photocatalytic oxidation of gas-phase acetaldehyde in the application of indoor air purification. The mica/TiO 2 /Fe 2 O 3 -x (MTF-x, x = m Fe2O3 : m TiO2 = 0.5–2: 100) composites were synthesized by a sol-gel assisted hydrothermal method. The MTF-1.5 composite shows optimal photocatalytic performance, which is 1.8 times photodegradation efficiency and 2.2 times CO 2 mineralization efficiency higher than those of pure TiO 2 . The enhanced photocatalytic performance of MTF-x (x = 0.5–2) composites could be associated with enhanced reflectivity of mica, which eventually improved the light absorption properties. Also, the presence of TiO 2 /Fe 2 O 3 heterostructure facilitated charge separation in the MTF ternary composite. Besides, superoxide radical was proven as the decisive active species for the degradation of gaseous acetaldehyde. This work provides a systematic approach to develop a potential multi-functional pearlescent pigment to purify indoor air.

研究领域: 材料科学 · 环境科学 · 化学工程
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