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ADVANCED FUNCTIONAL MATERIALS · 2025 · IF 19

A Self-Detection Mechanism Toward Stable Multiple Perception of Ionic Skins

Shuting Shen,Chengfei Liu,Wenxin Fan,Kunyan Sui

Ionic skins (I-skins) hold significant potential for mimicking the complex sensory functions of human skin. However, they suffer from unstable sensing performance because the water content and temperature of I-skins are susceptible to the surrounding environment. Here, a self-detection sensing mechanism designed to address this critical issue, ensuring stable perception of multiple stimuli in I-skins, is introduced. It is demonstrated that gradient polyelectrolyte (GP) conductors possess two parameters—resistance and self-induced potential—that are responsive to temperature and water content. Through establishing the functional relations of resistance and potential against temperature and water content based on the Nernst−Planck and Arrhenius equations, respectively, the temperature and water content of resulting GP I-skins can be self-detected/calculated in real-time from the measured resistance and potential signals. Such self-detection capability allows GP I-skins not only to self-calibrate their sensing parameters for accurate detection of mechanical stimuli across varying environmental conditions but also to discern surrounding temperature and humidity in accordance with Flory−Rehner theory. This self-detection sensing mechanism offers a powerful tool for developing I-skins capable of stable perception of multiple stimuli in changing environments without complex and undesired encapsulation.

CAS / MDL: 7727-54-0 110-18-9
研究领域: 材料科学 · 生物医学工程
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Materials Horizons · 2018 ·Vol. 6 ·期 3 ·538-545 · IF 13.183

Adaptable polyionic elastomers with multiple sensations and entropy-driven actuations for prosthetic skins and neuromuscular systems

Zhouyue Lei,Peiyi Wu

A novel type of adaptable polyionic elastomers with rational molecular design is reported to address the dilemma encountered in soft electronic and ionic conductors. The conductivity of these elastomers is stable both during stretching and in air. The polyionic elastomers are highly transparent, 3D-printable, ultra-stretchable, self-healable, self-powered, and capable of sensing strain, stress, touch, humidity, temperature, etc. In addition, they can mimicking organisms with entropy-driven actuation and feedback. This type of materials contributes to prosthetic skins and neuromuscular systems and shows great potential for soft robotics and artificially intelligent applications.

研究领域: 材料科学 · 生物医学工程 · 人工智能
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