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Journal of Cleaner Production · 2023 · IF 11.1

Synergistic assisted hydrogen production of tailings slurry and coal slurry: Process and mechanism investigation

Keheng Pan,Jijia Deng,Guangfei Qu,Kunling Wei,Yuqi Liang

This study investigated the process and mechanism of synergistically assisted hydrogen production from tailings and coal slurry. We have identified the optimal tailings as lead-zinc tailings through experimentation with different tailings mixed with pulverized coal . Furthermore, we have analyzed the electrochemical properties of Fe 2+ and Fe 3+ at different concentration gradients in a hydrochloric acid environment and our results have confirmed that the presence of Fe 3+ in the simplified environment does not affect the electrochemical processes . to determine the respective roles and effects of the extract and residue of the lead-zinc tailings slurry with equal amounts of coal dust added to them, which has confirmed that it is the lead-zinc tailings extract that has the primary influence. In addition, the electrocatalysis of Fe 3+ in the presence of both lead-zinc tailings and coal results in a small increase in current density, and the improvement in current density due to direct and indirect oxidation of coal particles is also extremely limited. Based on our analysis, we have concluded that the increase in current density brought about by the synergistic hydrogen production from lead-zinc tailings-supported coal is mainly due to the different oxidation processes of Fe 2+ .

研究领域: 环境科学 · 能源科学 · 电化学
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