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INDUSTRIAL CROPS AND PRODUCTS · 2024 · IF 5.6

Cotton fiber-based composite aerogel derived from waste biomass for high-performance solar-driven interfacial evaporation

Mingyuan Liu,Xinyang He,Jiatai Gu,Zhen Li,Huijie Liu,Wendi Liu,Yue Zhang,Maorong Zheng,Jianyong Yu,Liming Wang,Xiaohong Qin

Cellulose-based composite aerogels derived from natural fibers have attracted widespread attention in the emerging field of solar-driven interfacial evaporation to produce clean water in an eco-friendly manner. However, the complex extraction process of cellulose and the expensive photothermal materials are urgent challenges for the preparation of solar-driven interfacial evaporators, which seriously hinder real applications. In this paper, the high-performance composite aerogel-based evaporators that could be directly constructed from cotton staple fibers derived from waste cotton fabrics without the cellulose extraction process and the photothermal conversion materials produced from the carbonization of waste cotton straw were reported. With the help of excellent hydrophilicity, water conductivity, and light capturing, the evaporators achieved outstanding light absorptivity (95.6%) and stable water evaporation rate (1.96 kg·m −2 ·h −1 ) under one sun irradiation. In the long-term practical application, the obtained evaporator exhibited excellent durability and recyclability, which facilitated the continuity of the evaporation process. Furthermore, the solar-driven interfacial evaporator was employed to purify seawater and various kinds of wastewater containing methyl orange (MO), indigo (ID), and acid black (AB). Interestingly, the evaporator could realize stable power generation due to the formation of an ionic gradient during the simulated seawater desalination, with an output voltage of 139 mV under one sun irradiation. The cotton fiber-based composite aerogels designed in this study have the advantages of cleanliness and high efficiency, which occupy significant economic value and extensive application potential in the fields of actual water purification and green energy development.

研究领域: 材料科学 · 环境科学 · 能源科学
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Journal of the Taiwan Institute of Chemical Engineers · 2019 · IF 3.834

In-suit preparation of CdSe quantum dots/porous channel biochar for improving photocatalytic activity for degradation of tetracycline

Qiuyue Men,Tao Wang,Changchang Ma,Lili Yang,Yang Liu,Pengwei Huo,Yongsheng Yan

In this paper, a simple in-suit method was used to load CdSe quantum dots (QDs) onto HTC (abbreviated as Hydrothermal biochar, HTC) to form CdSe/HTC composites. Fourier transform infrared spectrometer and X-ray photoelectron spectroscopy were used to detect and analyze the surface valence and composition of CdSe/HTC composites. The photocatalytic degradation activity was judged by photodegrading tetracycline (TC). Compared with pure CdSe quantum dots, the best photocatalytic degradation efficiency of CdSe/HTC complex containing 15% HTC was 73%, which was attributed to the high carrier transport efficiency of HTC and the inhibition reorganization of photogenerated electron-hole pairs. More importantly, the hydrothermal biochar used in this paper was extracted from waste biomass and had the characteristics of economy, environmental protection and high utilization rate, and was in line with the basic viewpoint of sustainable use of resources.

研究领域: 环境科学 · 材料科学
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