ADVANCED FUNCTIONAL MATERIALS
·
2021
·Vol. 31
·期 15
·2009580
·
IF 18.808
Guowei Xiong,Yuke Chen,Ziqian Zhou,Fan Liu,Xiaoyu Liu,Linjing Yang,Qilu Liu,Yuanhua Sang,Hong Liu,Xiaoli Zhang,Jin Jia,Weijia Zhou
Electrocatalytic water splitting for the production of hydrogen proves to be effective and available. In general, the thermal radiation synthesis usually involves a slow heating and cooling process. Here, a high-frequency induction heating (IH) is employed to rapidly prepare various self-supported electrocatalysts grown on Ni foam (NF) in liquid- and gas-phase within 1–3 min. The NF not only serves as an in situ heating medium, but also as a growth substrate. The as-synthesized Ni nanoparticles anchored on MoO 2 nanowires supported on NF (Ni-MoO 2 /NF-IH) enable catalysis of hydrogen evolution reaction (HER), showing a low overpotential of −39 mV (10 mA cm −2 ) and maintaining the stability of 12 h in alkaline condition. Moreover, the NiFe layered double hydroxide (NiFe LDH/NF-IH) is also synthesized via IH and affords outstanding oxygen evolution reaction (OER) activity with an overpotential of 246 mV (10 mA cm −2 ). The Ni-MoO 2 /NF-IH and NiFe LDH/NF-IH are assembled to construct a two-electrode system, where a small cell voltage of ≈1.50 V enables a current density of 10 mA cm −2 . More importantly, this IH method is also available to rapidly synthesize other freestanding electrocatalysts on NF, such as transition metal hydroxides and metal nitrides.
研究领域:
材料科学
·
能源化学
✓ 已验证
DOI
高影响因子
PROGRESS IN ORGANIC COATINGS
·
2023
·
IF 6.6
Potao Sun,Chaolu Niu,Wenxia Sima,Tao Yuan,Ming Yang,Mingke Zhao,Zheng Fang,QiChang Liu,Qin Deng
Polymer insulation materials are subjected to a combination of electromagnetic fields, mechanical stresses, long-term light exposure, ambient temperature and other operating conditions that produce mechanical and electrical tree damage which lead to insulation failure. Self-healing technology is a fundamental solution to this problem. However, effective long-term self-healing of mechanical and electrical tree damage to insulating materials is extremely challenging. To address this issue, this work reports a magnetic field dual responsive blueberry-like microsphere (MFDR-BLMS) that makes a breakthrough in the long-term self-healing of mechanical and electrical damage. The microspheres are attracted to the vulnerable area of the insulating material by the directional magnetic field. When the damage come into contact with the microspheres, the high thermal conductivity microspheres as a whole rapidly melt and fill the damage channels under the action of electromagnetic induction heating. This method achieves a magnetically dual-action, non-contact, long-term effective self-healing of mechanical and electrical tree damage after photothermal aging of insulation materials. This is expected to eliminate the requirement for human contact during the repair process under live conditions and provides a new technological idea for the industrial application of self-healing materials for electrical insulation.
研究领域:
材料科学
·
电气工程
✓ 已验证
产品关联
DOI
高影响因子
Coatings
·
2023
·Vol. 13
·期 9
·1531
·
IF 3.4
Jie Pang,Wenfeng Qin,Wentao You,Mian Zhong,Qing’an Meng
Ice accumulation on the surface of aircraft is a serious threat to flight safety and a fatal factor causing air accidents. However, traditional aircraft deicing methods no longer meet the requirements of safe flight due to changes in aircraft structural materials. In recent years, the application of carbon fiber-reinforced polymer (CFRP) materials in the aviation structure industry has increased. In this study, we demonstrate an economical, easy-to-prepare, and pollution-free approach to deice an aircraft through induction heating. The nickel-coated carbon fiber-reinforced polymer used as the induction heater for aircraft deicing is obtained by electroless nickel plating on the surface of the CFRP. The result shows that it takes just 110 s to achieve a temperature of 205 °C on the nickel-plated CFRP when the input voltage is 30 V, as well as melting the ice layer with a thickness of 30 mm, while the temperature of this material can reach up to 81 °C by electric heating when the input voltage is 1.5 V. Meanwhile, the nickel-plated CFRP exhibits good repeatability during the induction heating. Based on the excellent electrothermal properties, the nickel-plated CFRP polymer shows a prominent deicing ability, which provides a promising strategy for the deicing of aircraft.
研究领域:
材料科学
·
航空航天工程
✓ 已验证
产品关联
DOI
高影响因子
JOURNAL OF FOOD ENGINEERING
·
2020
·
IF 4.499
Gaoshang Wang,Zhili Wan,Xiaoquan Yang
It is a challenge to pasteurize higher-viscosity and heat-sensitive foodstuffs via traditional convective heat transfer. Herein, we demonstrate the potential application of magnetic induction heating (MIH) as a novel uniform heating method applied in the pasteurization of liquid whole eggs (LWEs). Upon exposure to an alternating magnetic field (AMF), the magnetic microbeads with a large size (50 μm) generated heat via the magnetic hysteresis effect, providing accurate and homogeneous heating due to the high specific absorption rate (SAR) of 3108.4 ± 30.6 W/(g Fe) and a homogeneous particle dispersion in high-viscosity food media. A 7.6 log reduction of Salmonella Enteritidis could be achieved in LWEs treated by MIH at 68 °C and 60 s, which was comparable to the inactivation performance of the convective heating protocol at 60 °C and 210 s (6.0 log reduction). Importantly, MIH showed a critical temperature-time regime to prevent the coagulation of egg proteins, thus maintaining the quality attributes associated with fresh LWEs. The obtained results suggested that MIH could be a potential alternative to conventional convective heating for pasteurization applications.
研究领域:
食品科学
·
微生物学
✓ 已验证
产品关联
DOI
高影响因子
ACS Applied Materials & Interfaces
·
2019
·
IF 8.456
Yingle Tao,Guoshun Huang,Qiangqiang Li,Qiannan Wu,Haiqing Li
Based on carbon fibers (CFs) delivered localized electrical induction heat, a novel electrical induction framework synthesis (EIFS) strategy has been developed to in-situ grow versatile metal–organic frameworks (MOFs) on CFs, resulting in the production of a set of MOF-coated CF (MOF@CF) fibers. Detailed studies on the production of UiO-66-NH2@CFs indicate that the use of EIFS leads to dramatically accelerated MOF growth at dozen times higher reaction rate than that of the conventional solvothermal reaction. By periodically switching anodes during EIFS reactions, uniform MOF@CF fibers with well-controlled MOF loadings have been achieved depending on the reaction conditions. Mediated by the embedded CFs in the resulting MOF@CFs, MOF@CFs exhibit well-regulated electrical induction heating capacities depending on MOF loadings and the applied voltages. Driven by such localized heat, up to 100% of the adsorbed CO2 in UiO-66-NH2@CF can be rapidly released, demonstrating an electrical induction framework regeneration (EIFR) process for highly efficient regeneration of MOFs. As CFs enable to rapidly deliver localized electrical induction with over 90% of electrothermal conversion efficiency and at rather low operation voltage, currently developed EIFS and EIFR process provide a highly efficient, low-energy, low operation cost, and safe way to highly efficient synthesis and regeneration of MOF materials.
研究领域:
材料科学
·
化学工程
✓ 已验证
DOI
PubMed
高影响因子
JOURNAL OF HAZARDOUS MATERIALS
·
2024
·
IF 12.2
Kai Yu,Yuxuan Tu,Mao Wan,Yongliang Guo,Shiqi Liu,Huimin Li,Yanchun Fan,Gang Zhao,Songxiong Zhong,Cun Liu,Xubiao Luo
Individual application of sulfide modification and electromagnetic field (EMF) can enhance the reactivity of nanoscale zero-valent iron (nZVI), yet the potential of both in combination is not clear. This work found that the reactivity of nZVI towards decabromodiphenyl ether was significantly enhanced by the combined effect of sulfidation and EMF. The specific reaction rate constant of nZVI increased by 7 to 10 times. A series of characterization results revealed that the sulfidation level not only affects the inherent reactivity but also the magnetic-induced heating (MIH) and corrosion (MIC) of nZVI. These collectively influence the degradation efficiency of nZVI under EMF. Sulfidation generally diminished the MIH effect. The low degree of sulfidation (S/Fe = 0.1) slightly reduced the MIC effect by 21.4%. However, the high degree of sulfidation (S/Fe = 0.4) led to significantly enhanced MIC effect by 107.1%. For S/Fe = 0.1 and 0.4, the overall enhancement in the reactivity resulting from EMF was alternately dominated by the contributions of MIH and MIC. This work provides valuable insights into the MIH and MIC effects about the sulfidation level of nZVI, which is needed for further exploration and optimization of this combined technology.
研究领域:
环境科学
·
材料科学
✓ 已验证
产品关联
DOI
PubMed
高影响因子
Coatings
·
2022
·Vol. 12
·期 3
·329
·
IF 3.236
Rong Tu,Chengyin Liu,Qingfang Xu,Kai Liu,Qizhong Li,Xian Zhang,Marina L. Kosinova,Takashi Goto,Song Zhang
SiC epitaxial wafers offer enormous potential for a wide range of telecom technologies due to their excellent properties. The experimental process was simulated by software, and the contour of gas flow velocity and raw material mass fraction inside the chamber were obtained. SiC films were epitaxially grown on 4H-SiC single crystalline substrates at different temperatures for one batch, using SiCl4, CH4, and H2as precursors. With increasing temperature, the crystal phase changed from 4H-SiC at 1773 K to a mixture of 4H- and 3C-SiC, and then a mixture of 3C-SiC and graphite at higher than 1923 K. The film was mainly (004)-oriented 4H-SiC and (111)-oriented 3C-SiC.Keywords:SiC film;high-frequency induction-heated halide CVD;crystalline phases distribution;microstructure;orientation
研究领域:
材料科学
·
半导体物理
✓ 已验证
产品关联
DOI
高影响因子
ACS Nano
·
2024
·
IF 15.8
Zhihui Lei,Shun Chen,Yu Liao,Wendong Liu,Lian Zhou,Benwei Fu,Peng Tao,Wen Shang,Jie Liu,Cuilan Hou,Chengyi Song,Tao Deng
In this study, we investigate the magnetic induction heating induced in a conducting polymer (CP) under alternative magnetic fields (AMFs). Experimental results and numerical simulations have proved that the magneto-thermal conversion of the CP is caused by the induced eddy current, which is related to the shape and intensity of the applied external AMF, and the intrinsic electrical conductivity, macrostructure and microstructure of the CP. By employing various fabrication methods, specific temperature distribution and control of thermal field within conducting polymer films and aerogels could be achieved. To exploit the potential of magnetic induction heating in CP for biomedical applications, we designed a conducting polymer aerogel-based self-adaptive heat patch and demonstrated its AMF-enabled localized heating of skin. In addition to the thermal ablation of tumor cells via magneto-thermal conversion of the CP, the promotion of neuronal differentiation at mild temperature by noninvasive magneto-electrical stimulation has also been demonstrated to be an effective strategy for tissue engineering.
研究领域:
材料科学
·
生物医学工程
·
组织工程
✓ 已验证
DOI
PubMed
高影响因子
CHROMATOGRAPHIA
·
2018
·Vol. 81
·期 7
·1043-1051
·
IF 1.401
Zhao Aixia,Xu Zhiqiang,Ma Liyi,Tian Zhenfeng,Gan Wuer
We report on the synthesis of Fe 3 O 4 @SiO 2 nanoparticles incorporated poly(divinylbenzene) monolithic column via in situ polymerization. The monolith had larger specific surface area and relatively uniform porous structure and was characterized by scanning electron microscopy, nitrogen adsorption–desorption, and Fourier transform infrared spectroscopy. The monolith was then applied for the evaluation of gas chromatography separation properties. Here, an electromagnetic induction heating technique was employed to control the column temperature with the thermal effect of eddy current in ferromagnetic materials Fe 3 O 4 . The monolith offered good separation efficiency for benzene and toluene and a higher column efficiency was obtained up to 4481 and 9216 plates per meter, respectively. In addition, the injection volume and column capacity of the proposed system are as much as 5 µL and 100 ng. This makes it possible to use a UV detector. The fabricated Fe 3 O 4 @SiO 2 nanoparticles incorporated poly(divinylbenzene) monolithic column has been shown to be very promising for gas chromatography separation. Graphical Abstract
研究领域:
分析化学
·
材料科学
✓ 已验证
产品关联
DOI
高影响因子
Advanced Science
·
2022
·Vol. 10
·期 3
·2204840
·
IF 17.521
Yifeng Ying,Guifang Yang,Yingle Tao,Qiannan Wu,Haiqing Li
Sorption-based atmospheric water harvesting (AWH) offers a promising solution to the water scarcity in arid regions. However, majority of the existing AWH sorbents are suffering from rather poor water productivity due to their slow water adsorption–desorption cycling capability especially when they are applied in high packing thickness. Herein, an oxygen plasma-treated magnetic flower-like porous carbon (P-MFPC) with large open surfaces, abundant surface oxygen-containing moieties, and excellent localized magnetic induction heating (LMIH) capacity is developed. These merits, together with the use of air-blowing-assisted water adsorption and LMIH-driven water desorption strategy, synergistically allow P-MFPC with 2 cm of packing thickness to complete a AWH cycling in 20 min and deliver a record 4.5 L H2O kg −1 day −1 of water productivity at 30% relative humidity. Synergistically enabling such an ultrafast AWH cycling at high sorbent packing thickness provides a promising way for the scalable high-yield AWH with compact AWH systems.
研究领域:
材料科学
·
环境科学
✓ 已验证
DOI
PubMed
高影响因子
CARBON
·
2023
·
IF 10.9
Jianhao Chen,Hongyi Liu,Fuyong Wang,Hao-Fan Wang,Yonghai Cao,Hongjuan Wang,Xixian Yang,Hao Yu
Organic pollutants have become an urgent problem for human health and the ecological system. The development of a multifunctional and efficient catalyst is of great significance for environmental governance. However, the catalytic conversion process of organic pollutants requires a large amount of energy, and traditional energy supply may further exacerbate environmental pollution. Herein, we propose an integrated magnetic material system that can serve as a magnetic heating medium to provide energy and as catalyst to promote the catalytic reaction . Iron-encapsulated carbon nanotubes activate peroxomonosulfate to generate active free radicals, achieving nearly complete degradation of the organic pollutant Orange II. The reaction exhibits excellent stability and repeatability, which may be attributed to the heating method applied to the magnetic sites, allowing the iron-encapsulated carbon nanotubes to maintain a stable structure. Further loading with Ag allows the catalyst to achieve near 100 % conversion of formaldehyde in air. This study aims to provide an effective and green strategy for environmental pollution treatment by integrating magnetic induction heating and catalytic conversion technology.
研究领域:
环境科学
·
材料科学
✓ 已验证
产品关联
DOI
高影响因子
Materials Science & Engineering C-Materials for Biological Applications
·
2016
·
IF 3.42
Huan Zhou,Saisai Hou,Mingjie Zhang,Mengmeng Yang,Linhong Deng,Xinbo Xiong,Xinye Ni
In present work condensed phosphates (P 2 O 7 4 − and P 3 O 10 5 − ) were used as phosphate source in induction heating to deposit calcium phosphate coatings. The phase, morphology, and composition of different phosphate-related coatings were characterized and compared using XRD, FTIR, and SEM analyses. Results showed that P 2 O 7 4 − formed calcium pyrophosphate hydrate coatings with interconnected cuboid-like particles. The as-deposited calcium tripolyphosphate hydrate coating with P 3 O 10 5 − was mainly composed of flower-like particles assembled by plate-like crystals. The bioactivity and cytocompatibility of the coatings were also studied. Moreover, the feasibility of using hybrid phosphate sources for preparing and depositing coatings onto magnesium alloy was investigated.
研究领域:
材料科学
·
生物材料
·
表面工程
✓ 已验证
DOI
PubMed
高影响因子
危险品化学品经营许可证（带存储）