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JOURNAL OF COLLOID AND INTERFACE SCIENCE · 2024 · IF 9.4

Ionic fuel-powered hydrogel actuators for soft robotics

Ting Zhao,Yu Tan,Yitan Li,Xu Wang

Hypothesis Hydrogel actuators powered by chemical fuels are pivotal in autonomous soft robotics. Nevertheless, chemical waste accumulation caused by chemical fuels hampers the development of programmable and reusable hydrogel actuating systems. We propose the concept of ionic fuel-powered soft robotics which are constructed by programmable salt-responsive actuators and use waste-free ionic fuels. Experiments Herein, soft hydrogel actuators were developed by orchestrating the Janus bilayer hydrogels’ capacity for swelling and shrinking. Decomposable and easily removable ionic fuels were applied to power the actuators. Swelling tests were used to evaluate the deformability of the hydrogels. Tensile tests were performed to investigate the modulus of the hydrogels. The bonded interface composed of the interpenetrating polymer chains from both hydrogel layers bilayer was evidenced by the optical microscopy and scanning electron microscopy. The ionic conductivities of solutions were determined by a conductivity meter. Furthermore, a range of biomimetic soft robots with various shapes and asymmetrical structures have been designed and fabricated to execute complex functions. Findings The programmable actuators powered by ionic fuel exhibit adjustable bending orientations, amplitudes, and durations, along with consistent cyclic actuations enabled by replenishment of the fuel without noticeable loss in performance. Many life-like programmable soft robotic systems were designed, indicating spatiotemporally controllable functions.

研究领域: 材料科学 · 软体机器人学 · 生物工程
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