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Green Energy & Environment · 2023 · IF 13.3

Temperature-regulation liquid gating membrane with controllable gas/liquid separation

Baiyi Chen,Huimeng Wang,Jiadai Xu,Liting Pan,Yuan Jing,Xu Hou

Membrane separation technology with the ability to regulate gas/liquid transport and separation is critical for environmental fields, such as sewerage treatment, multiphase separation, and desalination. Although numerous membranes can dynamically control liquid-phase fluids transport via external stimuli, the transport and separation of gas-phase fluids remains a challenge. Here, we show a temperature-regulation liquid gating membrane that allows in-situ dynamically controllable gas/liquid transfer and multiphase separation by integrating a thermo-wettability responsive porous membrane with functional gating liquid. Experiments and theoretical analysis have demonstrated the temperature-regulation mechanism of this liquid gating system, which is based on thermo-responsive changes of porous membrane surface polarity, leading to changes in affinity between the porous membrane and the gating liquid. In addition, the sandwich configuration with dense Au-coated surfaces and heterogeneous internal components by a bistable interface design enables the liquid gating system to enhance response sensitivity and maintain working stability. This temperature-regulation gas/liquid transfer strategy expands the application range of liquid gating membranes, which are promising in environmental governance, water treatment and multiphase separation.

CAS / MDL: 20769-85-1 156-57-0
研究领域: 环境工程 · 材料科学 · 化学工程 · 膜技术
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