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Advanced Materials Technologies · 2020 ·Vol. 5 ·期 9 ·2000262 · IF 5.969

Deep-Learning-Enabled MXene-Based Artificial Throat: Toward Sound Detection and Speech Recognition

Yukun Jin,Bo Wen,Zixiong Gu,Xiantao Jiang,Xiaolan Shu,Zhenping Zeng,Yupeng Zhang,Zhinan Guo,Yun Chen,Tingting Zheng,Yutao Yue,Han Zhang,Huijun Ding

Wearable sound detectors require strain sensors that are stretchable, sensitive, and capable of adhering conformably to the skin, and toward this end, 2D materials hold great promise. However, the vibration of vocal cords and muscle contraction are complex and changeable, which can compromise the sensing performance of devices. By combining deep learning and 2D MXenes, an MXene-based sound detector is prepared successfully with improved recognition and sensitive response to pressure and vibration, which facilitate the production of a high-recognition and resolution sound detector. By training and testing the deep learning network model with large amounts of data obtained by the MXene-based sound detector, the long vowels and short vowels of human pronunciation are successfully recognized. The proposed scheme accelerates the application of artificial throat devices in biomedical fields and opens up practical applications in voice control, motion monitoring, and many other fields.

CAS / MDL: 67-68-5 7664-39-3
研究领域: 生物医学工程 · 材料科学 · 人工智能
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Smart Materials and Structures · 2017 ·Vol. 26 ·期 9 ·095033 · IF 2.909

Flexible and wearable electronic silk fabrics for human physiological monitoring

Cuiping Mao,Huihui Zhang,Zhisong Lu

The development of textile-based devices for human physiological monitoring has attracted tremendous interest in recent years. However, flexible physiological sensing elements based on silk fabrics have not been realized. In this paper, ZnO nanorod arrays are grown in situ on reduced graphene oxide-coated silk fabrics via a facile electro-deposition method for the fabrication of silk-fabric-based mechanical sensing devices. The data show that well-aligned ZnO nanorods with hexagonal wurtzite crystalline structures are synthesized on the conductive silk fabric surface. After magnetron sputtering of gold electrodes, silk-fabric-based devices are produced and applied to detect periodic bending and twisting. Based on the electric signals, the deformation and release processes can be easily differentiated. Human arterial pulse and respiration can also be real-time monitored to calculate the pulse rate and respiration frequency, respectively. Throat vibrations during coughing and singing are detected to demonstrate the voice recognition capability. This work may not only help develop silk-fabric-based mechanical sensing elements for potential applications in clinical diagnosis, daily healthcare monitoring and voice recognition, but also provide a versatile method for fabricating textile-based flexible electronic devices.

研究领域: 生物医学工程 · 材料科学 · 传感器技术
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ACS Applied Materials & Interfaces · 2024 · IF 8.3

Bubbles-Induced Porous Structure-Based Flexible Piezoresistive Sensors for Speech Recognition

Xiaoguang Gao,Lin Yuan,Chengzhen Xue,Xiaoliang Zhang,Xuejuan Meng,Xiaochun Li

Flexible piezoresistive sensors with a porous structure that are used in the field of speech recognition are seldom characterized by both high sensitivity and ease of preparation. In this study, a piezoresistive sensor with a porous structure that is both highly sensitive and can be prepared by using a simple method is proposed for speech recognition. The preparation process utilizes the interaction of bubbles generated by ethanol evaporation and active agents with polydimethylsiloxane to produce a porous flexible substrate. This preparation process requires neither templates nor harsh experimental conditions such as a low temperature and a low pressure. Furthermore, the prepared piezoresistive sensor has excellent properties, such as a high sensitivity (27.6 kPa–1), a satisfactory response time (800 μs), and a good stability (10,000 cycles). When used for speech recognition, more than 1500 vocalizations and silent speech signals obtained from subjects saying numbers from “0” to “9” were collected by the sensor for training a convolutional neural network model. The average accuracy of the recognition reached 94.8%. The simple preparation process and the excellent performance of the prepared flexible piezoresistive sensor endow it with a wide application prospect in the field of speech recognition.

CAS / MDL: 68-12-2
研究领域: 材料科学 · 电子工程 · 人工智能
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CHEMICAL ENGINEERING JOURNAL · 2024 · IF 13.3

Multi-functional MXene/helical multi-walled carbon nanotubes flexible sensor for tire pressure detection and speech recognition enabled by machine learning

Chunqing Yang,Dongzhi Zhang,Weiwei Wang,Hao Zhang,Lina Zhou

Flexible sensors exhibit exceptional mechanical adaptability, enabling them to accommodate diverse operational settings. They seamlessly conform to the deformation requirements of the human body or irregular object surfaces and have found extensive applications in human motion tracking, tire pressure monitoring, and human–computer interactions. Here, we have prepared a sandwich-structured MXene/helical multi-walled carbon nanotubes (Hs-MWCNTs) flexible strain sensor. The fabricated sensor has a wide detection range (0–77 %), high sensitivity (gauge factor 243.6 at 70–77 % strain), reliable repeatability (over 35000 s), and other excellent sensing performance. MXene/Hs-MWCNTs flexible strain sensor has significant advantages in detecting tiny signals such as human pulse and tire pressure. The constructed 4 × 4 flexible sensing arrays can achieve pressure distribution detection of objects with different shapes. In addition, based on MXene/Hs-MWCNTs flexible strain sensor and continuous wavelet transform convolutional neural network algorithms, speech recognition of some English words is successfully achieved with a recognition accuracy of 94.4 %. The results indicate that MXene/Hs-MWCNTs flexible strain sensor has great potential for application in fields such as human motion detection, health monitoring and speech recognition.

CAS / MDL: 308068-56-6 7647-01-0
研究领域: 材料科学 · 传感器技术 · 机器学习
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Advanced Science · 2025 · IF 14.1

Piezoresistive Effect: A New Concept for Hearing Aids

Mengyao Gao,Weijie Liu,Kun Chen,Huili Sun,Xiaoqing Liu,Haonan Xing,Huatang Wang,Benpeng Zhu,Haizhong Guo

Hearing loss is among the most prevalent sensory impairments globally. Hearing aids assist individuals with hearing impairments in perceiving sound more effectively, serving as essential tools for reconnecting them with the world. Herein, an MXene/Polyvinyl Alcohol sound sensor (MPSS) capable of recognizing weak sound signals is developed. It can not only recognize different speech signals and sound properties but also show good stability in the process of long-term sound recording. In addition, by combining the sensor with machine learning, the accuracy rate of voiceprint recognition of wildlife conservation is up to 99%, underscoring its practical significance for wildlife protection. Utilizing piezoresistive effects, a hearing aid with a detection sound threshold of 60 dB and a frequency range of 20–4000 Hz is achieved, which provides a feasible scheme in hearing aids.

CAS / MDL: 7789-24-4
研究领域: 生物医学工程 · 材料科学 · 人工智能
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Materials · 2025 ·Vol. 18 ·期 9 ·2014 · IF 3.2

Anti-Freezing Conductive Ionic Hydrogel-Enabled Triboelectric Nanogenerators for Wearable Speech Recognition

Tao Chen,Andeng Liu,Wentao Lei,Guoxu Wu,Jiajun Xiang,Yixin Dong,Yangyang Chen,Bingqi Chen,Meidan Ye,Jizhong Zhao,Wenxi Guo

Flexible wearable electronics face critical challenges in achieving reliable physiological monitoring, particularly due to the trade-off between sensitivity and durability in flexible electrodes, compounded by mechanical modulus mismatch with biological tissues. To address these limitations, we develop an anti-freezing ionic hydrogel through a chitosan/acrylamide/LiCl system engineered via the solution post-treatment strategy. The optimized hydrogel exhibits exceptional ionic conductivity (24.1 mS/cm at 25 °C) and excellent cryogenic tolerance. Leveraging these attributes, we construct a gel-based triboelectric nanogenerator (G-TENG) that demonstrates ultrahigh sensitivity (1.56 V/kPa) under low pressure. The device enables the precise capture of subtle vibrations at a frequency of 1088 Hz with a signal-to-noise ratio of 16.27 dB and demonstrates operational stability (>16,000 cycles), successfully differentiating complex physiological activities including swallowing, coughing, and phonation. Through machine learning-assisted analysis, the system achieves 96.56% recognition accuracy for five words and demonstrates good signal recognition ability in different ambient sound scenarios. This work provides a paradigm for designing environmentally adaptive wearable sensors through interfacial modulus engineering and ion transport optimization.

CAS / MDL: 9012-76-4
研究领域: 材料科学 · 生物医学工程 · 传感器技术
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LANGMUIR · 2023 · IF 3.9

Tendon-Inspired Anisotropic Hydrogels with Excellent Mechanical Properties for Strain Sensors

Huijuan Lin,Rui Wang,Shengnu Xu,Xiangye Li,Shasha Song

Anisotropic conductive hydrogels mimicking the natural tissues with high mechanical properties and intelligent sensing have played an important role in the field of flexible electronic devices. Herein, tensile remodeling, drying, and subsequent ion cross-linking methods were used to construct anisotropic hydrogels, which were inspired by the orientation and functionality of tendons. Due to the anisotropic arrangement of the polymer network, the mechanical performance and electrical conductivity were greatly improved in specific directions. The tensile stress and elastic modulus of the hydrogel along the network orientation were 29.82 and 28.53 MPa, which were higher than those along the vertical orientation, 9.63 and 11.7 MPa, respectively. Moreover, the hydrogels exhibited structure-dependent anisotropic sensing. The gauge factors (GFs) parallel to the prestretching direction were greater than the GF along the vertical direction. Thus, the tendon-inspired conductive hydrogels with anisotropy could be used as flexible sensors for joint motion detection and voice recognition. The anisotropic hydrogel-based sensors are highly expected to promote the great development of emerging soft electronics and medical detection.

CAS / MDL: 79-10-7 79-06-1 110-26-9
研究领域: 生物材料学 · 柔性电子学 · 医学检测
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Nano-Micro Letters · 2024 ·Vol. 17 ·期 1 ·1-15 · IF 31.6

Ti3C2Tx Composite Aerogels Enable Pressure Sensors for Dialect Speech Recognition Assisted by Deep Learning

Xiao Yanan,Li He,Gu Tianyi,Jia Xiaoteng,Sun Shixiang,Liu Yong,Wang Bin,Tian He,Sun Peng,Liu Fangmeng,Lu Geyu

Emphasized the innovation in both the material design and methodology between the sensing performance and mechanical properties. The composite aerogel pressure sensors exhibited low hysteresis (13.69%), wide detection range (6.25 Pa-1200 kPa), and cyclic stability to acquire stable and accurate pronunciation signals. Over 6888 and 4158 pronunciation signals were collected by the pressure sensor and utilized for training the convolutional neural network model, allowing for accurate recognition of six dialects (96.2% accuracy) and seven words (96.6% accuracy).

研究领域: 生物医学工程 · 传感器技术 · 人机交互 · 语音信号处理 · 功能材料 · 可穿戴设备
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JOURNAL OF COLLOID AND INTERFACE SCIENCE · 2025 · IF 9.7

Enhanced-performance flexible pressure sensors enabled by synergistic effect of hierarchical porous structures for motion sensing and deep learning-assisted speech recognition

Weiwei He,Puye Zhang,Zhonglue Hu,Shuai Yang,Wei Chen,Tianlong He,Lei Tang,Jiajia Zheng,Runsheng Li,Boce Xue,Guoqing Hu,Yanzhen Zhang

Amid the global wave of intelligentization, flexible pressure sensors have emerged as core sensing components owing to their excellent flexibility, portability, and highly sensitive response to pressure signals in fields such as human-computer interaction, health monitoring, smart wearable devices, and artificial-intelligence terminals. Herein, we developed a flexible pressure sensor with a hierarchically porous structure via a hybrid manufacturing strategy integrating three-dimensional (3D) printing and electrospinning. A MXene/silver nanowires/polydimethylsiloxane (MAP) conductive ink modified with nano silicon dioxide (SiO 2 ) was formulated to optimize printability, and the multi-scale porous sensing unit was constructed by direct ink writing (DIW) combined with a sacrificial template method, followed by encapsulation with a fibrous film electrode. Benefiting from the synergistic effect of macro-micro porous structure and the structural-mechanical matching design, the sensor exhibits high sensitivity (0.813 kPa −1 ), fast response (37 ms/30 ms), and an extremely low detection limit (1.47 Pa), thus enabling the effective monitoring of various human physiological motion signals and demonstrating significant potential in health monitoring applications. Furthermore, by integrating deep learning algorithms, high-accuracy recognition (94.9 %) of several spoken phrases is achieved, extending the sensor's applicability to human-computer interaction and intelligent speech perception. In summary, this study proposes a strategy based on a hybrid manufacturing technology for fabricating hierarchically porous flexible pressure sensors, demonstrating broad application prospects in health monitoring and smart human-computer interaction, thus providing new pathways for the innovative design and functional expansion of wearable electronic devices.

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Advanced Electronic Materials · 2025 · IF 5.3

MXene Aerogel Pressure Sensor Improved by Introducing Intermolecular Forces for Human Motion Detection and Voice Recognition

Anqi Zhou,Wenchang Yi,Yingjun Wu,Ziyi Wu,Yawei Fu,Tang Liu,Huimin Li,Naizheng Bian,Song Liu

MXene aerogels, known for their exceptional conductivity, hold significant potential in the development of pressure sensors. However, the van der Waals forces that solely exist between pure MXene nanosheets are inadequate for forming aerogels with high elasticity and mechanical properties, thus restricting the broad application of MXene aerogels in sensor technology. In this research, reduced graphene oxide (RGO) is utilized as the primary framework and incorporate polyaniline (PANI) to enhance intermolecular interaction forces, employing freeze-drying techniques to fabricate 3D porous-structured MXene aerogels. This approach significantly enhances the elasticity and electrical responsiveness of the aerogel. The resulting aerogel-based pressure sensor exhibits high sensitivity (4 kPa −1 ), a wide linear response range (1–20 kPa), rapid response/recovery time (300/100 ms), and excellent stability. The sensor is capable of detecting a variety of pressure signals, from gentle breezes to human motion, and is applied in voice recognition. Using a machine learning framework based on feature engineering, it is possible to accurately identify and classify distinctly pronounced letters from sensor outputs with an accuracy rate as high as 98%. In summary, the high-performance flexible pressure sensor based on MXene aerogel shows great potential for applications in health monitoring, smart wearable devices, and artificial intelligence.

研究领域: 材料科学 · 传感器技术 · 纳米技术 · 柔性电子学 · 人工智能
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Journal of Materials Chemistry A · 2022 ·Vol. 10 ·期 30 ·16297-16308 · IF 14.511

Ultrafast dynamic response of waterproof stretchable strain sensors based on wrinkle-templated microcracking

Lele Li,Yang Zheng,Enping Liu,Juanjuan Wang,Xue Han,Shichun Jiang,Fan Xu,Yanping Cao,Conghua Lu

Stretchable strain sensors simultaneously featuring a fast dynamic response, waterproof ability and a wide working strain range are highly required in practical applications. Here, we report a new class of high-performance strain sensors based on a wrinkle-templated microcracking mechanism involved in a strain-sensing bilayer configuration. Besides high stretchability, the resulting strain sensors with surface hierarchical micro/nanostructures have waterproof properties, ultrafast dynamic sensing behaviors (response time: ∼0.08 ms) and ultrahigh sensitivity in the whole strain range. As demonstrated, the waterproof stretchable strain sensor has outstanding capability such as in vibration monitoring and voice recognition with a frequency up to 20 000 Hz, and as dynamic-sensing electronic skins even under harsh conditions (e.g., underwater and small and large strains simultaneously loaded). The wrinkle-templated microcracking mechanism offers a simple general guideline to design diverse microcracking-based stretchable devices with highly boosted performances.

研究领域: 材料科学 · 传感器 · 纳米技术 · 电子学
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ADVANCED FUNCTIONAL MATERIALS · 2025 · IF 19

Switchable, Recyclable, and Time-Programmable Hydrogels via Counterion-Engineered Differential Metal-Ion Coordination

Kewei Zhao,Xianglei Zhao,Xin Guo,Yanyan Zhao,Mingqiong Tong,Lin Chen,Shujuan Zhuang,Xiangling Gu

Multifunctional hydrogels applied in flexible electronics and smart sensing face prominent challenges including functionality integration, environmental adaptability, and sustainability. This paper presents an anti-ion-regulated differential metal-ion coordination strategy to fabricate a multifunctional hydrogel (SP-M n+ X y− ) with switchable modules, recyclability, and time-dependent encryption. The SA-PAM double-network hydrogel, modulated by Fe 3+ and Ca 2+ (with Cl − or Ac − as counterions), exhibits distinct coordination behaviors: Fe 3+ demonstrates strong coordination due to high charge density, while Ca 2+ ’s binding is counterion-dependent–rapid network densification with CaCl 2 (fully dissociated Cl − ) versus controlled release with CaAc 2 (weakly dissociated Ac − ). The hydrogel achieves outstanding mechanical strength (0.52 MPa), wide sensing range (300%), fast response (114 ms), and freeze resistance (−20 °C). Reversible chelation of ethylene diamine tetraacetic acid enables efficient switching among conductive, adhesive, and sensing modules (performance decay < 17.95% after cycles). Leveraging Fe 3+ /Ca 2+ coordination kinetics, time-dependent color changes enable dynamic encryption. With high conductivity (15.1 S·m −1 ) and self-adhesion (9.5 kPa), the hydrogel serves as a wearable sensor for motion tracking, speech recognition, and electrocardiograph monitoring. Key innovations are achieved in this work, including: anti-ion-mediated precise property control, green fabrication of recyclable, multi-modal hydrogels, and kinetic-driven encryption, which advances hydrogel design for flexible electronics, sensing, and information security. Graphical Counterion-Mediated Differential Metal Coordination enables recyclable, multifunctional hydrogels (SP-M n+ X y− ) with switchable conductive/adhesive/sensing modules and time-dependent encryption, which yields advancing wearable electronics with the capability of motion/speech/ECG monitoring, self-power supply, and secure time-dependent information coding.

研究领域: 材料科学 · 高分子化学 · 柔性电子器件 · 传感器技术 · 生物医学工程 · 信息安全
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