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Nature Communications · 2020 ·Vol. 11 ·期 1 ·1-10 · IF 12.121

Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring

Yu Dejian,Wang Peng,Cao Fei,Gu Yu,Liu Jiaxin,Han Zeyao,Huang Bo,Zou Yousheng,Xu Xiaobao,Zeng Haibo

Ensuring nuclear safety has become of great significance as nuclear power is playing an increasingly important role in supplying worldwide electricity. β-ray monitoring is a crucial method, but commercial organic scintillators for β-ray detection suffer from high temperature failure and irradiation damage. Here, we report a type of β-ray scintillator with good thermotolerance and irradiation hardness based on a two-dimensional halide perovskite. Comprehensive composition engineering and doping are carried out with the rationale elaborated. Consequently, effective β-ray scintillation is obtained, the scintillator shows satisfactory thermal quenching and high decomposition temperature, no functionality decay or hysteresis is observed after an accumulated radiation dose of 10 kGy (dose rate 0.67 kGy h −1 ). Besides, the two-dimensional halide perovskite β-ray scintillator also overcomes the notorious intrinsic water instability, and benefits from low-cost aqueous synthesis along with superior waterproofness, thus paving the way towards practical application.

研究领域: 材料科学 · 核物理 · 辐射检测
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