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JOURNAL OF ALLOYS AND COMPOUNDS · 2024 · IF 5.8

Magnetic and electrical properties of Co2Te3 single crystal

Wei-Bin Wu,Yuan-Qiao Chen,Qi-Ling Xiao,Jun-Yi Ge

The Co-Te system has become a prominent field of research in recent times. CoTe 2 is confirmed to be a Dirac semimetal, while Co 2 Te is predicted to host the quantum anomalous Hall effect. Here, we have successfully grown high-quality Co 2 Te 3 single crystals using the solid-state reaction method and have characterized them using the energy dispersive X-ray spectroscopy, the X-ray diffraction and Laue diffraction. The X-ray rocking curve with a full-width at half-maximum of 0.067° shows Co 2 Te 3 single crystals have good crystalline quality and mosaicity. Co 2 Te 3 single crystals possess a hexagonal structure with the space group of P 6 3 / mmc . Resistivity measurements reveal typical metallic behavior with a transition from Non-Fermi liquid to low-temperature Landau Fermi-liquid behavior around 50 K, which can be fitted by the parallel resistance model. Magnetic measurements show no obvious anisotropy between the in-plane and out-of-plane directions with the presence of a small magnetic hysteresis at 1.8 K. Furthermore, Co 2 Te 3 single crystals undergo a magnetic phase transition around 50 K and an antiferromagnetic transition modulated by the magnetic field below 8 K.

CAS / MDL: 13494-80-9
研究领域: 凝聚态物理 · 材料科学
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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA · 2022 ·Vol. 119 ·期 51 ·e2211193119 · IF 12.779

Two-dimensional quantum universality in the spin-1/2 triangular-lattice quantum antiferromagnet Na2BaCo(PO4)2

Jieming Sheng,Le Wang,Andrea Candini,Wenrui Jiang,Lianglong Huang,Bin Xi,Jize Zhao,Han Ge,Nan Zhao,Ying Fu,Jun Ren,Jiong Yang,Ping Miao,Xin Tong,Dapeng Yu,Shanmin Wang,Qihang Liu,Maiko Kofu,Richard Mole,Giorgio Biasiol,Dehong Yu,Igor A. Zaliznyak,Jia-Wei Mei,Liusuo Wu

An interplay of geometrical frustration and strong quantum fluctuations in a spin-1/2 triangular-lattice antiferromagnet (TAF) can lead to exotic quantum states. Here, we report the neutron-scattering, magnetization, specific heat, and magnetocaloric studies of the recently discovered spin-1/2 TAF Na2BaCo(PO4)2, which can be described by a spin-1/2 easy axis XXZ model. The zero-field neutron diffraction experiment reveals an incommensurate antiferromagnetic ground state with a significantly reduced ordered moment of about 0.54(2) μB/Co. Different magnetic phase diagrams with magnetic fields in the ab plane and along the easy c-axis were extracted based on the magnetic susceptibility, specific heat, and elastic neutron-scattering results. In addition, two-dimensional (2D) spin dispersion in the triangular plane was observed in the high-field polarized state, and microscopic exchange parameters of the spin Hamiltonian have been determined through the linear spin wave theory. Consistently, quantum critical behaviors with the universality class of d = 2 and νz = 1 were established in the vicinity of the saturation field, where a Bose–Einstein condensation (BEC) of diluted magnons occurs. The newly discovered quantum criticality and fractional magnetization phase in this ideal spin-1/2 TAF present exciting opportunities for exploring exotic quantum phenomena.

研究领域: 凝聚态物理 · 量子磁性 · 强关联电子系统 · 低维量子系统 · 中子散射 · 量子相变
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