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INTERNATIONAL JOURNAL OF FOOD PROPERTIES · 2023 · IF 2.9

VIS-NIR radiation properties of starchy and protein foods and their impacts on radiant heating effects

Wei Yang,Linshuang Long,Yanjun Sun,Fan Yang,Luo Zhang,Kai Xu,Hong Ye

Infrared heating has been widely used in food processing; however, there are few studies on the VIS-NIR radiation properties of food. We measured the radiation properties of starchy foods (potato, Chinese yam and sweet potato) and protein foods (beef tenderloin, pork tenderloin and chicken breast) and dispersions of starches and proteins before and after heat treatment in the 0.38–2.5 μm band. The results show that the radiation penetration depths (RPDs) of all tested foods are relatively high in the 0.6–1.3 μm band, with maximum values in the range of 4–8 mm. After heat treatment, the RPDs of starchy foods slightly increase, while those of protein foods decrease to approximately 1/2 of the original values. Comparative heating experiments of potato, Chinese yam and sweet potato heated by a halogen lamp (1.04 μm) and a carbon fiber lamp (1.76 μm) with peak wavelengths in and out of the 0.6–1.3 μm band, respectively, show that the foods heated by the halogen lamp have faster heating rates and more uniform temperature distributions. Because starchy and protein foods have high RPDs in the 0.6–1.3 μm band, the VIS-NIR radiation containing this band is expected to achieve rapid heating.

CAS / MDL: 9005-25-8
研究领域: 食品科学 · 生物物理学
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FUEL · 2022 · IF 8.035

Three-stage pretreatment of food waste to improve fuel characteristics and incineration performance with recovery of process by-products

Rui Li,Minghui Gong,Bernard Wiafe Biney,Kun Chen,Wei Xia,He Liu,Aijun Guo

As of 2020, the annual generation of municipal solid waste (MSW) in China has surged to 235.12 Mt, and food waste (FW) accounts for more than 60 %. The most common treatment method is incineration, which accounts for 62.13 %. This research proposes a three-stage pretreatment method for FW that is suitable for incineration while recovering by-products and energy from the pretreatment process. The first stage is dehydration; as compared to hot air drying (HAD) processes, freeze drying (FD) exhibits a higher dehydration and oil preservation rate, allowing for the preservation of organic matter content and the recovery of freshwater resources from FW. The second stage is oil recovery; the FW extracted oil (FWEO) can be used to produce biodiesel, and this stage also helps to improve the effectiveness of the subsequent torrefaction process. The third stage improves the energy and fuel characteristics of the organic residue of FW and enhances the combustion performance by optimizing the torrefaction temperature. The solid fuel obtained at a torrefaction temperature of 350 °C shows the best combustion performance, with a solid yield of 35.76 %, a torrefaction temperature of 300 °C might be chosen to further improve the solid yield.

CAS / MDL: 75-09-2 110-54-3 67-56-1
研究领域: 环境科学 · 能源工程 · 废物管理
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JOURNAL OF CHROMATOGRAPHY B-ANALYTICAL TECHNOLOGIES IN THE BIOMEDICAL AND LIFE SCIENCES · 2016 · IF 2.687

A reliable compound-specific nitrogen isotope analysis of amino acids by GC-C-IRMS following derivatisation into N-pivaloyl-iso-propyl (NPIP)esters for high-resolution food webs estimation

Zhongyi Zhang,Jing Tian,Hongwei Xiao,Nengjian Zheng,Xiaofei Gao,Renguo Zhu,Huayun Xiao

The signatures of natural stable nitrogen isotopic composition (δ 15 N) of individual amino acid (AA) have been confirmed to be a potentially effective tool for elucidating nitrogen cycling and trophic position of various organisms in food webs. In the present study, a two-stage derivatisation approach of esterification followed by acylation was evaluated. The biological samples underwent acid hydrolysis and the released individual AA was derivatived into corresponding N -pivaloyl-isopropyl (NPIP) esters for nitrogen isotopic analysis in gas chromatography-combustion-isotope ratio mass spectrometry (GC-C-IRMS). Usually, 13 individual AA derivatives were separated with fine baseline resolution based on a nonpolar gas chromatography column (DB-5   ms). The minimum sample amount required under the presented conditions is larger than 20   ngN on column in order to accurately determine the δ 15 N values. The δ 15 N values determined by GC-C-IRMS with a precision of better than 1‰, were within 1‰ after empirical correction compared to the corresponding measured by element analysis (EA)-IRMS. Bland-Altman plot showed highly consistency of the δ 15 N values determined by the two measurement techniques. Cation-exchange chromatography was applied to remove interfering fraction from the extracts of plant and animal samples and without nitrogen isotope fractionation during the treatment procedure. Moreover, this approach was carried out to estimate the trophic level of various natural organisms in a natural lake environment. Results highly proved that the trophic level estimated via the presented AA method well reflected the actual food web structure in natural environments.

研究领域: 生态学 · 分析化学
✓ 已验证 DOI PubMed 高影响因子
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Environmental Sciences Europe · 2024 ·Vol. 36 ·期 1 ·1-12 · IF 6

Bioaccessibility-corrected probabilistic health risk assessment of dietary metal(loid) exposure in six major food groups in children from Northwest China

Wang Beibei,Zhang Liwen,Feng Weiying,Zhang Han,Duan Xiaoli,Qin Ning

Dietary exposure to heavy metals and metalloids [metal(loid)s] deserves increased attention; however, there is a lack of a comprehensive understanding of the risks of dietary exposure from multi-type food intake and multi-metal(loid) exposure using a bioaccessibility-corrected method. Here, we determined the concentration and bioaccessibility of six toxic metal(loid)s in six major food groups in an industrial city with intensive smelting activity. By incorporating children’s dietary patterns, the probability distribution of health risks from dietary metal(loid)s exposure was assessed. Marked differences were observed in the dietary exposure characteristics within metal(loid)s and major food groups. Cereal and vegetables were the major food groups local children intake. Cereals, meat, beans, and aquatic products had the highest concentrations of Cu and Cd, Pb and Cr, Ni, and As, respectively. Generally, meat, eggs, and aquatic products exhibited higher bioaccessibility than cereals, beans, and vegetables. The bioaccessibility of metal(loid)s decreased in the following order: Pb > Cr > Cu > Ni > As > Cd. For non-carcinogenic risks, the average hazard index was 7.3, with 99.6% exceeding acceptable levels. Arsenic was the dominant risk element and aquatic product was the main risk source. The aggregated carcinogenic risk was 3.4 × 10–3, with Cr the major risk contributor and cereals and meat the dominant food sources. The findings demonstrated that (1) the metal(loid) dietary exposure risk of children from areas with intensive smelting activities should be taken seriously, and (2) it is necessary to identify the specific food category and metal(loid) based on a comprehensive analysis of the metal(loid) concentration and bioaccessibility, and dietary habits of the population to effectively reduce risk.

研究领域: 环境科学 · 公共卫生
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FOOD AND AGRICULTURAL IMMUNOLOGY · 2014 · IF 0.984

Development of a monoclonal antibody-based sandwich ELISA for the detection of ovalbumin in foods

Juan Peng,Xu Meng,Xiaofang Deng,Jianping Zhu,Hua Kuang,Chuanlai Xu

Hen egg is one of the most frequent causes of food allergy in infants and adults. Ovalbumin (OVA) has been identified as a major egg allergen. In order to detect OVA in foods, a highly sensitive sandwich enzyme-linked immunosorbent assay (ELISA) based on two monoclonal antibodies (mAbs) was established. The 2 mAbs were selected out of 17 murine hybridomas secreting OVA-specific antibody. Using mAb17 as the capture antibody and mAb15 as the detection antibody, the detection limit of the ELISA method was 0.51 ng/mL, and the linear dynamic range was between 1.95 and 500 ng/mL. The recovery ranged from 85.6 to 115.2%, whereas the intra- and inter-assay coefficients of variation were less than 8.6 and 13.9%, respectively. Sample analysis verified that the produced anti-OVA mAb and the developed ELISA may provide a valuable tool for the sensitive determination of OVA in processed foods and for future studies on the mechanism of how OVA functions in anaphylaxis.

CAS / MDL: 9003-99-0 54827-17-7
研究领域: 免疫学 · 食品科学 · 医学
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Food Analytical Methods · 2014 ·Vol. 7 ·期 9 ·1729-1736 · IF 1.802

Electrochemical Determination of Phoxim in Food Samples Employing a Graphene-Modified Glassy Carbon Electrode

Chao Mingyong,Chen Meifeng

Employing a graphene-modified glassy carbon electrode, a sensitive and convenient electrochemical method for the determination of phoxim by linear sweep voltammetry was developed. The electrochemical behavior of phoxim at the modified electrode was studied by cyclic voltammetry. In citric acid–phosphate buffers, the modified electrode exhibited excellent electrocatalytical effect on the reduction of phoxim and this was further used for the determination of phoxim. Under optimized analytical conditions, the reduction peak current showed a linear relationship with the concentration of phoxim in a range of 5.97 to 5,966 μg L −1 , with a correlation coefficient of 0.9993 and a detection limit of 2.39 μg L −1 . The proposed method shows excellent sensitivity, selectivity, and linearity and has been successfully applied for the determination of phoxim in a variety of food samples with satisfactory results.

CAS / MDL: 14816-18-3
研究领域: 分析化学 · 食品安全
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ENERGY CONVERSION AND MANAGEMENT · 2018 · IF 6.377

Microbial lipid production from food waste saccharified liquid and the effects of compositions

Xiaoyu Ma,Zhen Gao,Ming Gao,Yingqun Ma,Hongzhi Ma,Min Zhang,Yu Liu,Qunhui Wang

The residues of food waste after removing waste cooking oils could be converted to microbial lipid by oleaginous yeasts and microbial lipid could be used as a raw material of biodiesel with waste cooking oils. This process would have positive environmental and economic benefits. However, the composition of food waste is extremely complex. Many types of organic acids, such as lactic acid and acetic acid, could be accumulated during the collection, transportation and storage processes. The effects of these substances on microbial lipid production remained unknown. In this study, food waste saccharified liquid (FWSL) without any additional nutrients was fed to Rhodosporidium toruloides 2.1389 for microbial lipid production. Total biomass concentration, lipid concentration and lipid yield increased by 87.4%, 69.4% and 69.3%, respectively, compared with the YPD medium. Remarkably, increasing the concentration of lactic acid in the medium promoted the total biomass concentration of yeast. Furthermore, lipid concentration decreased slightly when single lactic acid or single acetic acid concentration was below 5 g/L or 1 g/L in the culture media. Metal elements that were present in the medium had considerable synergistic effects on lipid production. When four metal elements (i.e. Mg, Ca, Na and K) were present in the medium, total biomass concentration, lipid concentration, lipid content and lipid yield increased by 22.01%, 33.51%, 9.43% and 33.33%, respectively, compared with those in the control group. The interaction among the FWSL compositions that led to the promotion of microbial lipid production was beyond the inhibition effect. The engineering implication analysis evidently suggested that the process of microbial lipid production from FWSL was economically feasible and had potential industrial application prospects.

研究领域: 生物工程 · 环境科学
✓ 已验证 DOI 高影响因子
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ENERGY CONVERSION AND MANAGEMENT · 2024 · IF 9.9

Integrating photoenzymatic decarboxylation and anaerobic digestion to convert food waste into hydrocarbon: Performance and process intensification

Xiaobo Guo,Ao Xia,Feng Li,Yun Huang,Xianqing Zhu,Wuyuan Zhang,Xun Zhu,Qiang Liao

The integration of photoenzymatic decarboxylation and anaerobic digestion (AD) to convert food waste into hydrocarbon was conducted for the first time. The performance of fatty acid photodecarboxylase from Chlorella variabilis NC64A ( Cv FAP) was optimized in a biphasic system with petroleum ether as the oil phase; conversion of palmitic acid reached 42.2 % in 1 h, which was 26.4 times that in the single-phase catalysis. This biphasic system was further employed to convert the lipase hydrolysate of waste oil from food waste into hydrocarbon, where the production rate of C17 hydrocarbon was 1.7 mM/h. Meanwhile, the non-oil components from food waste were used in AD to generate C1 hydrocarbon methane. Adding magnetite increased the specific methane yield up to 154.0 % compared to the control group on day 22. The average hydrocarbon generation rate and energy production rate in photoenzymatic decarboxylation were 24.3 and 269 times those in AD, respectively.

研究领域: 环境生物学 · 生物化学
✓ 已验证 DOI 高影响因子
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ENVIRONMENTAL POLLUTION · 2017 · IF 5.099

Trophic predator-prey relationships promote transport of microplastics compared with the single Hypoaspis aculeifer and Folsomia candida

Dong Zhu,Qing-Fang Bi,Qian Xiang,Qing-Lin Chen,Peter Christie,Xin Ke,Long-Hua Wu,Yong-Guan Zhu

Although the roles of earthworms and soil collembolans in the transport of microplastics have been studied previously, the effects of the soil biota at different trophic levels and interspecific relationships remain poorly understood. Here, we examine three soil microarthropod species to explore their effects on the transport of microplastics. The selected Folsomia candida and Hypoaspis aculeifer are extensively used model organisms, and Damaeus exspinosus is a common and abundant indigenous species in China. A model food chain (prey-collembolan and predator-mite) was structured to test the role of the predator-prey relationship in the transport of microplastics. Commercial Polyvinyl chloride (PVC) particles (Diameter: 80–250 μm) were selected as the test microplastics, because large amounts of PVC have persisted and accumulated in the environment. Synchronized soil microarthropods were held in plates for seven days to determine the movement of microplastics. The 5000 microplastic particles were carefully placed in the center of each plate prior to the introduction of the animals. Our results clearly show that all three microarthropod species moved and dispersed the microplastics in the plates. The 0.54%, 1.8% and 4.6% of the added microplastic particles were moved by collembolan, predatory mite and oribatid mite, respectively. Soil microarthropods (<0.2 cm) transported microplastic particles up to 9 cm. The avoidance behavior was observed in the collembolans in respect of the microplastics. The predatory -prey relationship did promote the transport of microplastics in the plates, increasing transport by 40% compared with the effects of adding single species (P < .05). Soil microarthropods commonly occur in surface soils (0–5 cm) and, due to their small body size, they can enter soil pores. Our results therefore suggest that the movement of microplastics by soil microarthropods may influence the exposure of other soil biota to microplastics and change the physical properties of soils.

研究领域: 生态学 · 环境科学
✓ 已验证 DOI PubMed 高影响因子
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FOOD CONTROL · 2022 · IF 6.652

Nanobodies for accurate recognition of iso-tenuazonic acid and development of sensitive immunoassay for contaminant detection in foods

Feng Wang,Yuan-Yuan Yang,De-Bin Wan,Jia-Dong Li,Yi-Fan Liang,Zhen-Feng Li,Yu-Dong Shen,Zhen-Lin Xu,Jin-Yi Yang,Hong Wang,Jan Gettemans,Bruce D. Hammock,Yuan-Ming Sun

The accurate analysis of chemical isomers plays an important role in the study of their different toxic effects and targeted detection of pollutant isomers in foods . The Alternaria mycotoxins tenuazonic acid (TeA) and iso-tenuazonic acid (ITeA) are two isomer mycotoxins with the lack of single analysis methods due to the similar structures. Antibody-based immunoassays exhibit high sensitivity and superior application in isomer-specific determination. Previously, various kinds of antibodies for TeA have been prepared in our group. Herein, highly specific nanobodies (Nbs) against ITeA mycotoxin were selected from immune nanobody phage display library, and one of Nbs, namely Nb(B3G3) exhibited excellent affinity, thermal stability as well as organic solvent tolerance. By molecular simulation and docking technology, it was found that stronger interaction between Nb(B3G3) and ITeA lead to higher affinity than that for its isomer TeA. Furthermore, a sensitive indirect competitive enzyme-linked immunosorbent assay (icELISA) was established with a limit of detection (LOD) of 0.09 ng/mL for ITeA mycotoxin. The recovery rate of ITeA in spiked samples was analyzed with 84.8%–89.5% for rice, 78.3%–96.3% for flour, and 79.5%–90.7% for bread. A conventional LC-MS/MS method was used to evaluate the accuracy of this proposed icELISA, which showed a satisfactory consistent correlation. Since the convenient strategy for nanobody generation by phage display technology, this study provide new biorecognition elements and sensitive immunoassay for analysis of ITeA in foods.

研究领域: 食品安全 · 免疫学 · 分析化学
✓ 已验证 DOI PubMed 高影响因子
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Insects · 2021 ·Vol. 12 ·期 6 ·507 · IF 2.769

Effects of Different Nitrogen Sources and Ratios to Carbon on Larval Development and Bioconversion Efficiency in Food Waste Treatment by Black Soldier Fly Larvae (Hermetia illucens)

Yan Lu,Shouyu Zhang,Shibo Sun,Minghuo Wu,Yongming Bao,Huiyan Tong,Miaomiao Ren,Ning Jin,Jianqiang Xu,Hao Zhou,Weiping Xu

Simple SummaryBlack soldier fly larvae (BSFL) have received global research interest and industrial application due to their high performance on the organic waste treatment. However, the substrate C/N property, which may affect larvae development and the waste bioconversion process greatly, is significantly less studied. The current study focused on the food waste treatment by BSFL, compared the nitrogen supplying effects of 9 nitrogen species (i.e., NH4Cl, NaNO3, urea, uric acid, Gly, L-Glu, L-Glu:L-Asp (1:1,w/w), soybean flour, and fish meal), and further examined the C/N effects on the larval development and bioconversion process. We found that NH4Cl and NaNO3led to poor larval growth and survival, while 7 organic nitrogen species exerted no harm to the larvae. Urea was further chosen to adjust the C/Ns. Results showed that lowering the C/N from the initial 21:1 to 18:1–14:1 improved the waste reduction and larvae production performance, and C/N of 18:1–16:1 was further beneficial for the larval protein and lipid bioconversion, whereas C/N of 12:1–10:1 resulted in a significant performance decline. Therefore, the C/N range of 18:1–16:1 is likely the optimal condition for food waste treatment by BSFL and adjusting food waste C/N with urea could be a practical method for the performance improvement.AbstractBiowaste treatment by black soldier fly larvae (BSFL,Hermetia illucens) has received global research interest and growing industrial application. Larvae farming conditions, such as temperature, pH, and moisture, have been critically examined. However, the substrate carbon to nitrogen ratio (C/N), one of the key parameters that may affect larval survival and bioconversion efficiency, is significantly less studied. The current study aimed to compare the nitrogen supplying effects of 9 nitrogen species (i.e., NH4Cl, NaNO3, urea, uric acid, Gly, L-Glu, L-Glu:L-Asp (1:1,w/w), soybean flour, and fish meal) during food waste larval treatment, and further examine the C/N effects on the larval development and bioconversion process, using the C/N adjustment with urea from the initial 21:1 to 18:1, 16:1, 14:1, 12:1, and 10:1, respectively. The food wastes were supplied with the same amount of nitrogen element (1 g N/100 g dry wt) in the nitrogen source trial and different amount of urea in the C/N adjustment trial following larvae treatment. The results showed that NH4Cl and NaNO3caused significant harmful impacts on the larval survival and bioconversion process, while the 7 organic nitrogen species resulted in no significant negative effect. Further adjustment of C/N with urea showed that the C/N range between 18:1 and 14:1 was optimal for a high waste reduction performance (73.5–84.8%,p< 0.001) and a high larvae yield (25.3–26.6%,p= 0.015), while the C/N range of 18:1 to 16:1 was further optimal for an efficient larval protein yield (10.1–11.1%,p= 0.003) and lipid yield (7.6–8.1%,p= 0.002). The adjustment of C/N influenced the activity of antioxidant enzymes, such as superoxide dismutase (SOD,p= 0.015), whereas exerted no obvious impact on the larval amino acid composition. Altogether, organic nitrogen is more suitable than NH4Cl and NaNO3as the nitrogen amendment during larval food waste treatment, addition of small amounts of urea, targeting C/N of 18:1–14:1, would improve the waste reduction performance, and application of C/N at 18:1–16:1 would facilitate the larval protein and lipid bioconversion process.Keywords:nitrogen source;carbon to nitrogen ratio;food waste;urea;black soldier fly larvae;Hermetia illucens

研究领域: 环境科学 · 昆虫学 · 废弃物处理
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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY · 2019 · IF 4.084

Experimental study on the energy conversion of food waste via supercritical water gasification: Improvement of hydrogen production

Mi Yan,Hongcai Su,Dwi Hantoko,Ekkachai Kanchanatip,Fauziah Binti Shahul Hamid,Sicheng Zhang,Guobin Wang,Zhang Xu

In this study, the model food waste was gasified to hydrogen-rich syngas in a batch reactor under supercritical water condition. The model food consisted of rice, chicken, cabbage, and cooking oil. The effects of the main operating parameters including temperature (420–500 °C), residence time (20–60 min) and feedstock concentration (2–10 wt%) were investigated. Under the optimal condition at 500 °C, 2 wt% feedstock and 60 min residence time, the highest H 2 yield of 13.34 mol/kg and total gas yield of 28.27 mol/kg were obtained from non-catalytic experiments. In addition, four commercial catalysts namely FeCl 3 , K 2 CO 3 , activated carbon, and KOH were employed to investigate the catalytic effect of additives at the optimal condition. The results showed that the highest hydrogen yield of 20.37 mol/kg with H 2 selectivity of 113.19%, and the total gas yield of 38.36 mol/kg were achieved with 5 wt% KOH addition Moreover, the low heating value of gas products from catalytic experiments with KOH increased by 32.21% compared to the non-catalytic experiment. The catalytic performance of the catalysts can be ranked in descending order as KOH > activated carbon > FeCl 3  > K 2 CO 3 . The supercritical water gasification (SCWG) with KOH addition can be a potential applied technology for food waste treatment with production of hydrogen-rich gases.

CAS / MDL: 7705-08-0
研究领域: 能源转化 · 环境工程
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