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Soft Matter · 2022 ·Vol. 18 ·期 48 ·9197-9204 · IF 4.046

A strong and tough gelatin/polyvinyl alcohol double network hydrogel actuator with superior actuation strength and fast actuation speed

Shiyu Yao,Xingyue Sun,Lina Ye,Haiyi Liang

Hydrogels are widely used in actuators that are applied in numerous fields such as multifunctional sensors, soft robots, artificial muscles, manipulators and microfluidic valves, and yet their applications in soft robots and artificial muscles are often limited by low actuation strength and slow actuation speed. Here, we develop a hydrogel actuator with high actuation strength (contraction strength of 850 kPa), fast actuation speed (response time of 90 s) and high energy density (output working density of 72 kJ m−3) by introducing a storing–releasing elastic potential energy method into a double network hydrogel. The high actuation strength is owing to the double network hydrogel, which possesses a high elastic modulus of 1.3 MPa, fracture strength of 1.8 MPa, and fracture energy of 16 kJ m−2. The fast actuation speed is due to the storing–releasing elastic potential energy method, which stretches the hydrogel and locks the hydrogel at deformed shape under external stimuli to store the elastic potential energy and then makes the hydrogel contract rapidly under new stimuli to release the pre-stored energy. A capture actuator and a hand muscle actuator are fabricated to achieve strong and fast actuation. The hydrogel actuator has shown potential applications in soft robots and artificial muscles.

CAS / MDL: 9002-89-5
研究领域: 材料科学 · 软体机器人 · 生物医学工程
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ADVANCED MATERIALS · 2022 ·Vol. 35 ·期 9 ·2202193 · IF 32.086

High-Performance Organohydrogel Artificial Muscle with Compartmentalized Anisotropic Actuation Under Microdomain Confinement

Longhao Zhang,Hao Yan,JiaJia Zhou,Ziguang Zhao,Jin Huang,Lie Chen,Yunfei Ru,Mingjie Liu

Current hydrogel actuators mostly suffer from weak actuation strength and low responsive speed owing to their solvent diffusion-induced volume change mechanism. Here a skeletal muscle-inspired organohydrogel actuator is reported in which solvents are confined in hydrophobic microdomains. Organohydrogel actuator is driven by compartmentalized directional network deformation instead of volume change, avoiding the limitations that originate from solvent diffusion. Organohydrogel actuator has an actuation frequency of 0.11 Hz, 110 times that of traditional solvent diffusion-driven hydrogel actuators (<10 −3 Hz), and can lift more than 85 times their own weight. This design achieves the combination of high responsive speed, high actuation strength, and large material size, proposing a strategy to fabricate hydrogel actuators comparable with skeletal muscle performance.

研究领域: 材料科学 · 生物医学工程 · 仿生学
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