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Nano Research · 2021 ·Vol. 14 ·期 8 ·2846-2852 · IF 8.897

Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes

Wang Dongdong,Al-Mamun Mohammad,Gong Wanbing,Lv Yang,Chen Chun,Lin Yue,Wang Guozhong,Zhang Haimin,Zhao Huijun

The cyclopentanone and derivatives are a class of crucial fine chemicals for various industries and currently produced by conventional petrochemical synthetic routes. Here, we demonstrated a new synthetic approach to directly fabricate N-doped carbon nanotube (N-CNTs) networks with confined Co nanoparticles from Co 2+ -impregnated bulk g-C 3 N 4 as high performance hydrogenation rearrangement (HR) catalyst to efficiently convert a wide spectrum of biomass-derived furanic aldehydes to the corresponding cyclopentanones in water under a record-low H 2 pressure of 0.5 MPa and mild temperature. We unveiled a Co-catalysed bulk g-C 3 N 4 decomposition/carbonisation CNTs formation mechanism. A new HR pathway was also unveiled.

CAS / MDL: 1899-24-7 21921-76-6 120-92-3 96-41-3 930-30-3 141-78-6 98-01-1 1192-62-7 98-00-0 67-47-0 620-02-0 111-87-5 61305-27-9

研究领域: 催化 · 材料科学 · 化学工程 · 绿色化学

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