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Quasi-2D Mn3Si2Te6 Nanosheet for Ultrafast Photonics

Yan Lu,Zheng Zhou,Xuefen Kan,Zixin Yang,Haiqin Deng,Bin Liu,Tongtong Wang,Fangqi Liu,Xueyu Liu,Sicong Zhu,Qiang Yu,Jian Wu

The magnetic nanomaterial Mn3Si2Te6is a promising option for spin-dependent electronic and magneto-optoelectronic devices. However, its application in nonlinear optics remains fanciful. Here, we demonstrate a pulsed Er-doped fiber laser (EDFL) based on a novel quasi-2D Mn3Si2Te6saturable absorber (SA) with low pump power at 1.5 μm. The high-quality Mn3Si2Te6crystals were synthesized by the self-flux method, and the ultrathin Mn3Si2Te6nanoflakes were prepared by a simple mechanical exfoliation procedure. To the best of our knowledge, this is the first time laser pulses have been generated using quasi-2D Mn3Si2Te6. A stable pulsed laser at 1562 nm with a low threshold pump power of 60 mW was produced by integrating the Mn3Si2Te6SA into an EDFL cavity. The maximum power of the output pulse is 783 μW. The repetition rate can vary from 24.16 to 44.44 kHz, with corresponding pulse durations of 5.64 to 3.41 µs. Our results indicate that the quasi-2D Mn3Si2Te6is a promising material for application in ultrafast photonics.