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MnO2/AlOOH复合材料
INORGANIC CHEMISTRY · 2020 · IF 4.825

Highly Efficient MnO2/AlOOH Composite Catalyst for Indoor Low-Concentration Formaldehyde Removal at Room Temperature

Zhiyuan Liu,Jingpeng Niu,Weimin Long,Bing Cui,Kun Song,Fan Dong,Dong Xu

Indoor formaldehyde from substandard furniture and decorative materials seriously endangers human health. How to remove effectively indoor formaldehyde with low concentration at room temperature is a challenging problem. Using a MnO2/AlOOH composite by the MnO2 modification as a catalyst provides an effective approach to solve this challenge. Here, a new type of MnO2/AlOOH composite catalyst with high ability to remove indoor low-concentration formaldehyde was prepared by redox reaction at room temperature. A MnO2/AlOOH composite with a homogeneous dispersion of MnO2 has high specific surface area and a large amount of surface hydroxyl (−OH) which plays a major role in the adsorption of formaldehyde. A partially crystalline structure was observed in the composite, which contains multivalent Mn ions and a large number of vacancy defects. The surface −OH of composite shows strong oxidation activity through the charge exchange of multivalent Mn ions and vacancy defects. The composite has a higher ability to remove indoor low-concentration formaldehyde compared to the birnessite MnO2 at room temperature. This study proposes a new idea for the improvement of catalytic performance in the structure and composition of the catalyst.

研究领域: 环境科学 · 材料科学
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