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MnS-Mn3O4

JOURNAL OF THE ELECTROCHEMICAL SOCIETY · 2021 ·Vol. 168 ·期 11 ·116518 · IF 4.316

Communication—Partial Oxidation of MnS for Synergistic Electrocatalysis of N2-to-NH3 Fixation at Ambient Conditions

Peipei Li,Dan Cheng,Xiaohua Zhu,Meiling Liu,Youyu Zhang

Compared with the traditional Haber-Bosch process, electrochemical N2 to NH3 reduction affords an eco-friendly and sustainable alternative to ambient NH3 synthesis with the aid of efficient electrocatalysts. In this work, partial oxidation of MnS to obtain the MnS-Mn3O4 is proved as a promising noble-free electrocatalysts of N2 to NH3 fixation at ambient conditions. When tested in 0.1 M Na2SO4, the electrochemical N2 reduction reaction performance of MnS-Mn3O4 is improved comparing with the MnS, which achieves large NH3 yield of 16.74 μg h–1 mgcat.–1 and a high Faradaic efficiency of 5.72%. It also exhibits excellent selectivity of N2 to NH3 and strong long-term electrochemical stability.

CAS / MDL: 13446-34-9 7773-01-5 31175-20-9 13755-38-9 1313-82-2 68-04-2

研究领域: 化学 · 环境科学 · 材料科学

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