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Mo助剂

BIORESOURCE TECHNOLOGY · 2019 · IF 6.669

High performance of Mo-promoted Ir/SiO2 catalysts combined with HZSM-5 toward the conversion of cellulose to C5/C6 alkanes

Lele Jin,Wenzhi Li,Qiying Liu,Longlong Ma,Chao Hu,Ajibola T. Ogunbiyi,Mingwei Wu,Qi Zhang

In this study, the Mo-promoted Ir/SiO 2 (Ir-MoO x /SiO 2 ) catalysts combined with the zeolite HZSM-5 were used for the direct conversion of microcrystalline cellulose (MCC) to liquid fuel (C 5 /C 6 alkanes) in n-dodecane/H 2 O system. A synergistic effect was formed between the partially reduced MoO x species and the Ir particles, which effectively promoted the catalytic activity of Ir/SiO 2 catalyst. When the Mo/Ir molar ratio was 0.5, a high yield of C 5 /C 6 alkanes (91.7%) was achieved at 210 ℃ for 12 h. In addition, the main component of C 5 /C 6 alkanes was n-hexane, which was proven to be obtained by the hydrogenolysis of the key intermediate, sorbitol, formed from the hydrolysis and hydrogenation of MCC.

CAS / MDL: 98-86-2 50-70-4 110-82-7 9004-34-6 112-40-3 625-86-5 1003-38-9 93685-81-5 110-54-3 111-27-3 626-93-7 67-47-0 110802-84-1 623-37-0 652-67-5 96-37-7 107-83-5 78-78-4 96-14-0 590-36-3 71-41-0 584-02-1 109-66-0 56570-89-9

研究领域: 催化化学 · 能源化学

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