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NaTi2(PO4)3@碳

MATERIALS LETTERS · 2018 · IF 2.687

Facile synthesis of NaTi2(PO4)3-carbon composite through solid state method and its application in aqueous sodium ion battery

Xi Cao,Yang Yang

NASICON-structured NaTi 2 (PO 4 ) 3 is regarded as the most suitable anode for aqueous sodium ion batteries, however, the low electronic conductivity intrinsically restricts its application. NaTi 2 (PO 4 ) 3 -carbon composite is prepared by a facile solid state sintering method and studied as the anode in aqueous sodium ion battery , coupling with activated carbon as the cathode. This neutral sodium ion battery shows a high output voltage of 1.17 V, with outstanding rate and cycling stability. The full cell delivers an energy density of 33.4 Wh∙kg −1 at a power density of 33.4 W∙kg −1 based on the total active mass of the anode and cathode materials.

研究领域: 材料科学 · 电化学

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ELECTROCHIMICA ACTA · 2018 · IF 5.116

A long cycle-life Na-Mg hybrid battery with a chlorine-free electrolyte based on Mg(TFSI)2

Jing Zeng,Zulai Cao,Yang Yang,Yunhui Wang,Yueying Peng,Yiyong Zhang,Jing Wang,Jinbao Zhao

The commercial applications of rechargeable magnesium batteries (RMBs) are hindered by the slow diffusion kinetic of Mg 2+ ions in cathode materials. To overcome this problem, we design a new Na-Mg hybrid battery with the NaTi 2 (PO 4 ) 3 @Carbon (NTP@C) nanoparticles as a cathode material, the Mg metal as an anode and the Mg(TFSI) 2 + NaBH 4 - triglyme/1,2-Dimethoxyethane (DME) as a hybrid electrolyte. For the first time, the Mg(TFSI) 2 is applied as a Mg 2+ ions source in the chlorine-free Na-Mg hybrid electrolyte with NaBH 4 as both Na + ions source and moisture scavenger. The NTP@C/Mg hybrid battery shows excellent electrochemical performance. The corresponding average capacity decay after 1000 cycles is only 0.004% and 0.008% per cycle at 2 C and 10 C, respectively. Even at 20 C, about 60 mAh g −1 can be obtained after 26000 cycles. The impressive capacity retention of 93.7% and 90.2% can be obtained at 5 and 10 C, respectively. The excellent electrochemical performance of the hybrid battery confirms the feasibility using Mg(TFSI) 2 in the chlorine-free hybrid electrolyte for long term cycle. The developed NTP@C/Mg hybrid battery possesses the advantages of excellent electrochemical performances, good safety and low cost, making it promising for the commercial applications, especially for the large-scale energy storages.

CAS / MDL: 16940-66-2

研究领域: 材料科学 · 电化学

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