Organic Electrochemical Transistor with MoS2 Nanosheets Modified Gate Electrode for Sensitive Glucose Sensing

An organic electrochemical transistor (OECT) with MoS2nanosheets modified on the gate electrode was proposed for glucose sensing. MoS2nanosheets, which had excellent electrocatalytic performance, a large specific surface area, and more active sites, were prepared by liquid phase ultrasonic exfoliation to modify the gate electrode of OECT, resulting in a large improvement in the sensitivity of the glucose sensor. The detection limit of the device modified with MoS2nanosheets is down to 100 nM, which is 1~2 orders of magnitude better than that of the device without nanomaterial modification. This result manifests not only a sensitive and selective method for the detection of glucose based on OECT but also an extended application of MoS2nanosheets for other biomolecule sensing with high sensitivity.Keywords:organic electrochemical transistor;MoS2nanosheets;liquid phase ultrasonic exfoliation;glucose sensor