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An Endotenon Sheath-Inspired Double-Network Binder Enables Superior Cycling Performance of Silicon Electrodes

Journal 2022 · IF 23.655 · 14(1): 1-13 · 发表于 2022 年 4 月 1 日
作者: Jiang Meifang,Mu Pengzhou,Zhang Huanrui,Dong Tiantian,Tang Ben,Qiu Huayu,Chen Zhou,Cui Guanglei
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摘要

The double-network binder shows excellent adhesive and self-healing abilities, which help suppress electrode volume expansion and stabilize the electrode interface upon cycling. This binder induces a Li 3 N/LiF-rich solid electrolyte interface layer, which can suppress continuous electrolyte decomposition. Superior electrochemical performance can be achieved in Si/Li half cells and LiNi 0.8 Co 0.1 Mn 0.1 O 2 /Si full cells, even with a high loading of Si electrode.

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