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MXene-derived TiO2/MXene-loaded Ag for the degradation of the methyl orange

Journal 2021 · IF 3.089 · 36(24): 5002-5012 · 发表于 2021 年 12 月 2 日
作者: Zhou Haijun,Jiresse Nguetsa Kuate Loic,Zhang Weirun,Chen Zhengyang,Zhang Yamei,Zhang Jiaoxia
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摘要

The photodegradation technology can improve the status quo of environmental problems seriously which hindered the development and progress of human society. In this work, the two-dimensional transition metal carbide Ti 3 C 2 was prepared by HF etching of Ti 3 AlC 2 , and subsequently TiO 2 crystals were produced by hydrothermal method to prepare TiO 2 /Ti 3 C 2 composite. The Ag nanoparticles were then doped by photoreduction to form a ternary Ag/TiO 2 /Ti 3 C 2 composite. The effect of photocatalytic degradation of the methyl orange solution by Ag/TiO 2 /Ti 3 C 2 was investigated. The degradation only with Ag/TiO 2 /Ti 3 C 2 is worser than TiO 2 /Ti 3 C 2 , so H 2 O 2 was added to improve the catalytic ability and explore the photocatalytic mechanism. In 420 min, the degradation efficiency of methyl orange (MO) solution reached 71.09% due to the active-free radicals preventing the recombination of electron hole pairs to improve the catalytic performance of photocatalytic materials. Graphical abstract

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