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Bone-inspired MXene nano aerogels toward self-electricity generation and capacitive energy storage

Journal 2024 · IF 13.2 · 发表于 2024 年 10 月 28 日
作者: Yuan Yu,Menggang Li,Miao Sun,Zhaolin Yang,Yifan Liu,Senwei Hu,Jiazuo Zhou,Yudong Li,Haiyue Yang,Chengyu Wang
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摘要

The exceptional potential of MXene aerogels for practical applications is impeded by the energy-intensive processing and insufficient mechanical stability. Inspired by natural bones, herein, we report the MXene@regenerated nanocellulose aerogel (MRCA) with strong mechanical performance via dual aerogel fabrication to achieve high-performance energy generation and storage. The MRCA achieves a gravimetric capacitance of 1271.16 F g −1 at 2 mA cm −2 , and the energy density of the eco-friendly symmetrical MRCA-based solid-state supercapacitor reaches 0.11 mWh cm −2 , positioning it as a top contender among most state-of-the-art MXene-based electrodes. Additionally, the MRCA exhibits a robust specific tensile strength of 68.35 MPa cm 3 g −1 , resembling bone-like resilience. Therefore, MRCA can swiftly generate an open-circuit voltage of 181.24 V. The instant high voltage of MRCA transforms into diverse signals, driving MRCA-SC to release energy for electric devices in practical scenarios, paving the way for future sustainable power systems.

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