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Lattice Anchoring Stabilizes α-FAPbI3 Perovskite for High-Performance X-Ray Detectors

Journal 2025 · IF 36.3 · 18(1): 14 · 发表于 2025 年 7 月 29 日
作者: Huang Yu-Hua,Zou Su-Yan,Sheng Cong-Yi,Fang Yu-Chuang,Wang Xu-Dong,Wei Wei,Li Wen-Guang,Kuang Dai-Bin
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摘要

A lattice-anchoring strategy using low-dimensional perovskite addresses structural instability in α-formamidinium lead iodide (FAPbI 3 ) by matching crystal lattice, mitigating residual stress and tensile strain. Enhanced Pb-I bonding strength and reduced lattice strain improve structural stability and carrier mobility-lifetime product, enabling efficient charge transport. Optimized X-ray detectors achieve high sensitivity (1.83 × 10 5 μC Gy air –1 cm –2 ), low detection limit (27.6 nGy air s –1 ), and stable performance under prolonged irradiation.

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