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Topotactic fabrication of transition metal dichalcogenide superconducting nanocircuits

Journal 2023 · IF 16.6 · 14(1): 1-8 · 发表于 2023 年 7 月 18 日
作者: Wang Xiaohan,Wang Hao,Ma Liang,Zhang Labao,Yang Zhuolin,Dong Daxing,Chen Xi,Li Haochen,Guan Yanqiu,Zhang Biao,Chen Qi,Shi Lili,Li Hui,Qin Zhi,Tu Xuecou,Zhang Lijian,Jia Xiaoqing,Chen Jian,Kang Lin,Wu Peiheng
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摘要

Superconducting nanocircuits, which are usually fabricated from superconductor films, are the core of superconducting electronic devices. While emerging transition-metal dichalcogenide superconductors (TMDSCs) with exotic properties show promise for exploiting new superconducting mechanisms and applications, their environmental instability leads to a substantial challenge for the nondestructive preparation of TMDSC nanocircuits. Here, we report a universal strategy to fabricate TMDSC nanopatterns via a topotactic conversion method using prepatterned metals as precursors. Typically, robust NbSe 2 meandering nanowires can be controllably manufactured on a wafer scale, by which a superconducting nanowire circuit is principally demonstrated toward potential single photon detection. Moreover, versatile superconducting nanocircuits, e.g ., periodical circle/triangle hole arrays and spiral nanowires, can be prepared with selected TMD materials (NbS 2 , TiSe 2 , or MoTe 2 ). This work provides a generic approach for fabricating nondestructive TMDSC nanocircuits with precise control, which paves the way for the application of TMDSCs in future electronics.