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Energy-saving catalyst Fe/Ce-Mn-TiO2 for efficient low temperature NH3-SCR of NOx with high water content

Journal 2023 · IF 7.7 · 发表于 2023 年 6 月 26 日
作者: Chenhui Hu,Chunhong Liu,Kaimin Du,Chengkai Pang,Zuoxi Zhuo,Qiangsheng Gao
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摘要

An energy-saving catalyst 4%Fe/Ce-Mn-TiO 2 was prepared via a simple one-step impregnation-annealing process and used as a denitration catalyst at low temperature (≤180 °C) and high water content (∼20%). The results show that 4%Fe/Ce-Mn-TiO 2 catalyst exhibits good low-temperature catalytic activity and water resistance attributed to its highly dispersed metal oxide species, more surface-adsorbed oxygen and high stability of particles. The denitrification efficiencies of 4%Fe/Ce-Mn-TiO 2 catalyst are 90% (5% H 2 O) and 70% (20% H 2 O) at 170 ℃ respectively, which are superior to the commercial vanadium catalyst in service usually needs heating up to 220 ℃.