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In situ construction of an SnO2/g-C3N4 heterojunction for enhanced visible-light photocatalytic activity

Journal 2015 · IF 3.84 · 5(84): 68953-68963 · 发表于 2015 年 8 月 14 日
作者: Xi Chen,Banghong Zhou,Shuanglei Yang,Hanshuo Wu,Yuxin Wu,Laidi Wu,Jun Pan,Xiang Xiong
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摘要

Herein, a strong heterojunction, consisting of SnO2 nanoparticles grown on layered g-C3N4 nanosheets, was rationally designed and successfully synthesized via a facile hydrothermal method. The morphology, chemical structure, optical and electronic properties of the obtained SnO2/g-C3N4 hybrid nanocomposites were characterized. Furthermore, the photocatalytic activity of the novel photocatalysts was assessed. The results clearly indicate that the SnO2/g-CN-72.12% nanocomposite photocatalysts shows a stable cycle performance and exhibits significantly enhanced photocatalytic activity, which is 89 and 17 times higher than those of pure SnO2 and g-C3N4, respectively. The synergistic effect of the SnO2/g-C3N4 heterojunction can effectively accelerate the separation of photo-generated carriers and enhance the efficiency of interfacial charge transfer, which are proposed to be responsible for the enhancement of the photocatalytic activities. This study provides a low-cost and large-scale synthesis route for the production of visible light responsive photocatalysts that have potential in environmental purification applications.