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UV-assisted ultrafast construction of robust Fe3O4/polydopamine/Ag Fenton-like catalysts for highly efficient micropollutant decomposition

Journal 2021 · IF 7.963 · 发表于 2021 年 10 月 26 日
作者: Siyao Cheng,Xihao Pan,Cheng Zhang,Xiangpeng Lin,Qiu Zhuang,Yingzhi Jiao,Wei Dong,Xiaoliang Qi
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摘要

Fenton-like catalysts represent a family of promising materials to degrade micropollutants from contaminated water . However, the practical applications of Fenton-like catalysts are mainly limited by low catalytic degradation efficiency and stability. Herein, for the first time, rapid fabrication of Ag-decorated Fe 3 O 4 /polydopamine ( FPA ) microspheres was achieved via the help of UV irradiation, and the designed FPA microspheres were employed as Fenton-like catalysts to degrade micropollutants. Results showed that UV irradiation could activate the generation of the polydopamine shell and accelerate the Ag deposition, which played a crucial role in the rapid synthesis of highly active and stable FPA catalysts. Relative to reported catalysts, these FPA microspheres exhibited outstanding catalytic degradation performance, achieving 94.38% removal of tetracycline within 60 min. This work will provide a convenient strategy in the sustainable and efficient purification of wastewater to improve the quality of human life.