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Magnetic MoS2 nanosheets as recyclable solar-absorbers for high-performance solar steam generation

Journal 2020 · IF 6.274 · 发表于 2020 年 7 月 31 日
作者: Qingmiao Wang,Yi Qin,Feifei Jia,Yanmei Li,Shaoxian Song
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摘要

To deal with water scarcity, solar steam generation has been widely regarded as one of the promising methods for freshwater production. In this work, for the first time, a novel recyclable MoS 2 -based nanocomposite (magnetic MoS 2 nanosheets) was fabricated via the in-situ growth of nano Fe 3 O 4 on the polydopamine (PDA)-functionalized MoS 2 nanosheets , and subsequently applied as the solar absorber in the volumetric evaporation systems to generate solar steam. The magnetic MoS 2 nanosheets showed a superhigh solar absorption of over 96% within the whole wavelength range of 200–2500 nm. As a result, a high evaporation efficiency of 79.2% under the low illumination of 2.5 kW m −2 was achieved. In addition, the magnetic MoS 2 nanosheets not only showed the long-term well dispersion in aqueous solution due to the introduction of hydrophilic PDA, but also exhibited a fast and effective separation from aqueous solution with the help of the decorating nano Fe 3 O 4 , which much benefited to the continuously efficient solar steam generation and its good recyclability , respectively. Therefore, the MoS 2 -based nanomaterials in this work showed good prospects for solar energy harvesting .