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An approach for collaboratively separation and detection of uranium based on novel plastic scintillating resin

Journal 2024 · IF 8.1 · 发表于 2024 年 2 月 13 日
作者: Tianhao Dong,Xuan Jiang,Shan Xing,Yichen Hu,Yun Zhou,Yifan Li,Kesheng Hu,Keliang Shi,Tonghuan Liu,Jiangang He,Xiaolin Hou,Junqiang Yang
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摘要

It is extremely significant to monitor the radioactive uranium during the process of nuclear energy mining and disposal because of its high levels of chemical and radiological toxicity. In this work, a novel uranium plastic scintillator resin (U-PSresin) was successfully synthesized by suspension polymerization and used to rapidly enrich and determine uranium by Liquid Scintillation Counting (LSC). The U-PSresin shows excellent irradiation stability, extremely appropriate adsorption capacity of U(VI) (9.35 mg/g), which is convenient for the accurate measurement of LSC. Meanwhile, U-PSresin has a deviation of less than 5 % in adsorption and measurement repeatability and can be utilized to accurately measure more than 1 mg of natural uranium after enrichment. For different types of spiked water samples, the measurement deviation of U-PSresin is less than 15 %. This work demonstrates that U-PSresin can selectively enrich and quantitatively measure uranium in an aqueous environment, showcasing its significant potential in nuclear emergency scenarios and environmental monitoring.