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New flexible CsPbBr3-based scintillator for X-ray tomography

Journal 2022 · IF 2.389 · 33(8): 1-11 · 发表于 2022 年 8 月 12 日
作者: Lü Zhi-Wei,Wei Gong-Xiang,Wang Han-Qiu,Guan Yu,Jiang Ning,Liu Yun-Yan,Li Zhao,Qin Hua,Liu Hui-Qiang
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摘要

The evolution of lead halide perovskites used for X-ray imaging scintillators has been facilitated by the development of solution-processable semiconductors characterized by large-area, flexible, fast photoresponse. The stability and durability of these new perovskites are insufficient to achieve extended computed tomography scanning times with hard X-rays. In this study, we fabricated a self-assembled CsPbBr 3 -based scintillator film with a flexible large-area uniform thickness using a new room-temperature solution-processable method. The sensitivity and responsivity of X-ray photon conversion were quantitatively measured and showed a good linear response relationship suitable for X-ray imaging. We also demonstrated, for the first time, that the self-assembled CsPbBr 3 -based scintillator has good stability for hard X-ray microtomography. Therefore, such an inexpensive solution-processed semiconductor easily prepared at room temperature can be used as a hard X-ray scintillator and equipped with flexible CsPbBr 3 -based X-ray detectors. It has great potential in three-dimensional high-resolution phase-contrast X-ray-imaging applications in biomedicine and material science because of its heavy Pb and Br atoms.