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Piezocatalytic performance difference of graphitic carbon nitride (g-C3N4) derived from different precursors

Journal 2022 · IF 2.719 · 发表于 2022 年 6 月 6 日
作者: Yuqiu Shao,Chengcan Liu,Huirong Ma,Jingjing Chen,Chenlong Dong,Dajian Wang,Zhiyong Mao
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摘要

In this paper, four types of graphitic carbon nitride (g-C 3 N 4 ) are prepared from different precursors by thermal polycondensation method and the piezocatalytic performance difference of the obtained g-C 3 N 4 materials are investigated in detail. g-C 3 N 4 derived from thiourea delivers best piezocatalytic performance basing on KMnO 4 reduction experiment and rhodamine B degradation experiment. According to the differences of piezocatalytic performance of these g-C 3 N 4 materials, effects of morphology, composition and defects on piezocatalytic performances are discussed. Reactive oxygen species (ROS) capture experiment showed that g-C 3 N 4 could produce ROS through piezoelectric effect and hydroxyl radical (•OH) played a major role in pollutant degradation.