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Additive-Stabilized Emission Centers for Blue Perovskite Light-Emitting Diodes

Journal 2023 · IF 9.5 · 发表于 2023 年 5 月 23 日
作者: Shibing Zou,Kezhou Fan,Zidan Liu,Ligang Yuan,Qixin Yin,Jinke Bai,Jiarong Wang,Jiong Li,Min Yang,Jianwu Wei,Liqin Wu,Shuang Xu,Qifan Xue,Jiangsheng Xie,Kam Sing Wong,Jianbin Xu,Keyou Yan
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摘要

The performance of the blue perovskite light-emitting diodes (PeLEDs) is limited by the low photoluminescence quantum yields (PLQYs) and the unstable emission centers. In this work, we incorporate sodium bromide and acesulfame potassium into a quasi-2D perovskite to control the dimension distribution and promote the PLQYs. Benefiting from the efficient energy cascade channel and passivation, the sky-blue PeLED has an external quantum efficiency of 9.7% and no shift of the electroluminescence center under operation voltages from 4 to 8 V. Moreover, the half lifetime of the devices reaches 325 s, 3.3 times that of control devices without additives. This work provides new insights into enhancing the performance of blue PeLEDs.