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Blackbody-Sensitive Uncooled Infrared Detector with Ultra-Broadband and Ultrafast Photoresponse Based on Te/WTe2 Heterostructure

Journal 2024 · IF 8 · 12(25): 2400776 · 发表于 2024 年 7 月 16 日
作者: Yu Yu,Zhiyuan Dai,Haibiao Guan,Ruowen Wang,Tao Ye,Yonghao Bu,Jie Deng,Mengdie Shi,Liaoxin Sun,Rui Xin,Tianxin Li,Haibo Shu,Xiaoshuang Chen,Jing Zhou
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摘要

Blackbody-sensitive uncooled infrared photodetectors with ultra-broadband and ultrafast photoresponse have a profound impact on many areas of modern science and technology. However, it is a big challenge for both traditional photodetectors and emerging low-dimensional ones to simultaneously have all the above characteristics. Here, this challenge is addressed by establishing a Te/WTe 2 heterostructure photodetector. The built-in field of the heterostructure and the crossing conduction and valence bands of WTe 2 jointly result in a high responsivity and a visible-to-long-wavelength-infrared photoresponse range. The peak responsivity (at the 3.3 µm wavelength) reaches 914 mA W −1 at zero bias and 8.51 A W −1 at 2 V bias. Further, the joint action coupled with the high mobility of Te and WTe 2 promotes the 3-dB bandwidth to 153 kHz. The self-powered blackbody responsivity and specific detectivity reach 235.7 mA W −1 and 1.1 × 10 8 cm Hz 1/2 W −1 , respectively. The former increases to 5.82 A W −1 at 1 V bias. Moreover, this device is polarization-sensitive with a contrast ratio of 2. This work reveals the potential of the Te/WTe 2 heterostructure for high-performance room-temperature infrared photodetectors.