JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
·
2019
·Vol. 31
·期 1
·677-683
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IF 2.195
Wang Jing,Shen Bowen,Zhu Kongjun,Qiu Jinhao
With the ever increasing requirements for the structural health monitoring systems, the deposition of the piezoelectric films on the metallic or structural materials has turned out to be an important issue. Pb(Mg, Nb)O 3 -PbTiO 3 films with different buffer layers, i.e., in situ NiO, pre-fabricated NiO and LaNiO 3 , were successfully deposited on the Ni foil via the chemical solution deposition. The crystal structures and electric performances showed evident dependence on the buffer layer. Pre-deposited NiO and LaNiO 3 efficiently prevented the diffusion and complex reactions occurring at the interface, offered abundant nucleation sites, and thus helped the formation of pure high-qualified perovskite PMN-PT films at higher annealing temperatures.
研究领域:
材料科学
·
物理学
✓ 已验证
DOI
高影响因子
CERAMICS INTERNATIONAL
·
2016
·
IF 2.758
Zhenzhen Song,Yongcheng Zhang,Chaojing Lu,Zhenmeng Ma,Zhenjia Hu,Lin Wang,Chao Liu
Relaxor ferroelectric 0.75(Pb 1–3 x /2 La x )(Mg 1/3 Nb 2/3 )O 3 -0.25(Pb 1–3 x /2 La x )TiO 3 (La 3+ :PMN-PT x /75/25, where x =2.8, 3.0, 3.5, and 4.0 mol% of La 3+ ) transparent ceramics were fabricated by the combination of oxygen atmosphere pressureless sintering and hot-pressing sintering process. The optical transmittances of above four ceramics are higher than 60% at the wavelength of 500–900 nm. La 3+ :PMN-PT 3.0/75/25 exhibits the highest transparency around 70% at 900 nm which is very close to the theoretical transmittance 71%. Each of the four ceramics exhibits the pure perovskite phases. They show fully dense microstructures and their relative densities are higher than 99.8%. The ferroelectric and dielectric measurements indicate that these four ceramics exhibit relaxation characteristics. With increasing La 3+ content, (200) peak in XRD patterns shifts to higher angles and the average grain size increases, while the temperature Tε max corresponding to the maximum ε r , the remanent polarizations P r and coercive fields E c decrease gradually.
研究领域:
材料科学
·
物理学
✓ 已验证
DOI
高影响因子
CERAMICS INTERNATIONAL
·
2021
·
IF 4.527
Ze Fang,Xue Tian,Fengji Zheng,Xiaodong Jiang,Wanneng Ye,Yalin Qin,Xiaoxiong Wang,Yongcheng Zhang
Piezoelectric materials are widely used in electromechanical energy conversion, such as in sensors, transducers, and self-powered materials. In this paper, the influence of the Sm doping content on the microstructure and ferroelectric , piezoelectric , dielectric , and field-induced strain properties of 0.70Pb(Mg 1/3 Nb 2/3 )O 3 -0.30PbTiO 3 (PMN-PT) ceramics was investigated. Sm-doped PMN-PT ceramics with both high piezoelectric properties ( d 33 ∼1406 pC/N) and a large electromechanical coupling coefficient ( k p ∼0.69) were synthesized. Based on their piezoelectric effect, a maximum output voltage of 31 V was achieved under external forces. The output voltages showed satisfactory stability, repeatability, and sensitivity under periodic external forces; hence, Sm-doped PMN-PT piezoelectric ceramics are potential candidates for energy conversion and signal monitoring.
研究领域:
材料科学
·
物理学
✓ 已验证
DOI
高影响因子
ACTA MATERIALIA
·
2024
·
IF 8.3
Qinghu Guo,Xiangyu Meng,Dongxu Li,Zhonghua Yao,Huajun Sun,Hua Hao,Hanxing Liu,Shujun Zhang
Electrostrictive materials play an important role in the development of high precision actuators, due to the advantages of high resolution, low power dissipation and fast response time. However, the practical application of electrostrictive materials has been hindered by their limited displacement output. To address this, we conducted a study where we doped Pb(Mg 1/3 Nb 2/3 )O 3 -PbTiO 3 (PMN-PT) ceramics with Nd 2 O 3 , aiming to significantly improve the electrostrictive effect by enhancing local structural heterogeneities that disrupt the formation of long-range ordered ferroelectric domains. We obtained an optimized electrostrictive strain of 0.231 % with negligible hysteresis at an electric field of 50 kV/cm in 4 %Nd-doped PMN-PT ceramic, surpassing the performance of state-of-the-art lead-based electrostrictive ceramics. Of particular significance is that a high electrostrictive coefficients M 33 = 12.2 × 10 −16 m 2 /V 2 , together with a high mechanical work density of 0.035 J/cm 3 and a low power dissipation of 14 %, was achieved under a mechanical prestress of 50 MPa and an electric field of 10 kV/cm. Additionally, this material exhibits excellent fatigue resistance , with less than 3 % variation over 10 6 operation cycles. All these findings position 4 %Nd-doped PMN-PT ceramics as a promising candidate for high-performance electromechanical actuator applications.
研究领域:
材料科学
·
工程学
✓ 已验证
DOI
高影响因子
Journal of Advanced Dielectrics
·
2023
·
IF 3.1
Chaofeng Wu,Wen Gong,Jinfeng Geng,Jianye Cui,Lipeng Mi,Jingkai Nie,Qiang He,Jiajiu Li,Fang-Zhou Yao
Mn O 2 -modified Pb 0 . 9 6 2 5 Sm 0 . 0 2 5 ( Mg 1 / 3 Nb 2 / 3 ) 0 . 7 1 Ti 0 . 2 9 O 3 ceramics were prepared via a solid-state reaction approach. Results of detailed characterizations revealed that the addition of Mn O 2 has influence on the grain size, and all samples exhibit a pure perovskite structure. As the content of manganese increases, the volume of tetragonal phase increases. The ceramics with 1.5 mol.% Mn O 2 show a high electro-strain of 0.151% at 2 kV/mm. Therefore, this study provides a new insight into the role of Mn O 2 addition in tailoring the electrical properties of the Sm-PMN-PT ceramics by acceptor doping.
研究领域:
材料科学
·
电子工程
✓ 已验证
产品关联
DOI
高影响因子
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
·
2024
·
IF 11.2
Ruigang Qiu,Feifei Guo,Jie Wu,Wenqiang Bai,Yifei Chen,Hongqiao Zhou,Wei Long,Xiaojuan Li,Pinyang Fang,Zhonghua Dai,Jie Dong,Zengzhe Xi
In this work, texturing is proposed to improve the piezoelectric response of PSN-PMN-PT ceramics. The PSN-PMN-PT textured ceramic with a Lotgering factor F 001 higher than 99% was synthesized by the liquid-phase-assisted template grain growth (TGG) method. The addition of CuO/B 2 O 3 sintering aids improves the BT templates induced grain orientation growth behavior significantly. In comparison with its random counterpart, the Cu/B-T textured ceramic exhibits a high Lotgering factor F 001 of 99% and significantly enhanced dielectric and piezoelectric responses: ε r ∼ 3100, tan δ ∼ 0.8%, d 33 ∼ 1030 pC N –1 , d 33 ⋅ g 33 ∼ 34.2 × 10 –12 m 2 N –1 , d 33 * ∼ 1490 pm V –1 @5 kV cm –1 , S max ∼ 0.26%@20 kV cm –1 and H s ∼ 8.5%. In the meantime, good temperature stability is observed in the Cu/B-T textured ceramic with a variation of d 33 *@20 kV cm –1 and annealed d 33 lower than 9.68% and 18.1% over a wide temperature range of 25–140 °C. This work shows that PSN-PMN-PT textured ceramic (Cu/B-T) has great potential for electromechanical device applications such as precision actuators, ultrasound transducers, and energy harvesters.
研究领域:
材料科学
·
电子工程
✓ 已验证
产品关联
DOI
高影响因子
CERAMICS INTERNATIONAL
·
2025
·
IF 5.6
Dejun Liang,Xiaojuan Li,Yufeng Pi,Chenchen Xin,Mingyong Ren,Wei Long,Jie Wu,Pinyang Fang,Feifei Guo,Aiguo He,Zengzhe Xi
In this study, anisotropy strategy was employed to effectively enhance the piezoelectric performance and energy harvesting capability of 6 Pb(Sc 1/2 Nb 1/2 )O 3 -61 Pb(Mg 1/3 Nb 2/3 )O 3 -33PbTiO 3 (Abb. 6PSN–61PMN–33PT) ceramics. A high crystallographic orientation (Lotgering factor F 001 exceeding 98.5 %) was obtained in 6PSN–61PMN–33PT textured ceramics using the template grain growth (TGG) method. The piezoelectric response of 6PSN–61PMN–33PT ceramics was significantly improved, while the dielectric constant ( ε r ) was reduced. Compared to random ceramics, the textured ceramics exhibited higher figure of merit ( d 33 × g 33 ), markedly enhanced electromechanical coupling factor ( k p ) and piezoelectric coefficient ( d 33 ). The optimal properties were obtained in 6PSN–61PMN–33PT textured ceramics with 1 wt% BaTiO 3 template: d 33 = 1179 pC/N, k p = 0.87, ε r = 2766， d 33 × g 33 = 5.67 × 10 −11 m 2 /N, dielectric loss tan δ about 0.56 %, mechanical quality factor Q m = 194, and piezoelectric strain constant d 33 ∗ = 1130 pm/V and maximum strain S = 0.23 % at 20 kV/cm. These results demonstrate that 6PSN–61PMN–33PT textured ceramics hold promising application potential in energy harvesters.
研究领域:
材料科学
·
功能陶瓷
·
压电器件
·
能量采集
·
先进制造
✓ 已验证
产品关联
DOI
高影响因子
Nanoscale
·
2025
·
IF 5.1
Weili Deng,Tingting Zhou,Wanghong Zeng,Zihan Wang,Yiheng Liu,Boling Lan,Shenglong Wang,Yong Ao,Yue Sun,Shuai Wang,Zhaoyu Li,Long Jin,Weiqing Yang
Wearable piezoelectric sensors have gained significant attention for real-time biomechanical monitoring, yet existing designs often face limitations in sensitivity, durability, and dynamic response. To address these challenges, we develop a wearable sensor utilizing gradient-architected CNT/PMN-PT/PVDF piezoelectric composites for continuous gait monitoring during weight-bearing walking. The sensor features a dual-filler gradient configuration within the poly(vinylidene fluoride) (PVDF) matrix, where strategically distributed carbon nanotubes (CNTs) and lead magnesium niobate-lead titanate (PMN-PT) ceramic particles synergistically enhance electromechanical coupling efficiency. The CNTs-enriched surface layer boosts polarization by facilitating charge injection efficiency, while the gradient-arranged PMN-PT fillers induce stress concentration, further amplifying the piezoelectric output. As a result, the sensor exhibits exceptional performance, with a decent piezoelectric coefficient (d33* = 40 pm/V) and high sensitivity (172 mV/N). Both experimental tests and finite element simulations validate the superior performance of this gradient structure, making it highly effective for real-time kinematic monitoring during weight-bearing walking. This composite-based sensor represents a promising advancement in wearable health technology, with immediate applications in clinical gait analysis, rehabilitation monitoring and sports injury prevention.
研究领域:
材料科学
·
生物医学工程
·
传感技术
·
柔性电子学
·
人体运动分析
✓ 已验证
产品关联
DOI
PubMed
高影响因子
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
·
2019
·
IF 4.029
Xudong Qi,Yan Zhao,Enwei Sun,Juan Du,Kai Li,Ye Sun,Bin Yang,Rui Zhang,Wenwu Cao
The photoluminescence , dielectric relaxation, ferroelectric hysteresis, and field-induced strain properties of Pr 3+ -doped 0.24Pb(In 1/2 Nb 1/2 )O 3 -0.42Pb(Mg 1/3 Nb 2/3 )O 3 -0.34PbTiO 3 (PIN-PMN-PT:Pr 3+ ) multifunctional ceramics have been investigated. It was found that Pr 3+ doping enhanced the dielectric diffuseness and relaxation behavior of PIN-PMN-PT ceramics. Slim P - E loops and S - E curves appear in PIN-PMN-PT:Pr 3+ ceramics when the Pr 3+ doping concentration reaches 1.4 mol%. Local domain configurations associated with phase transitions were investigated by piezoresponse force microscopy (PFM). Large electrostrictive coefficient Q 33 (˜0.03 m 4 /C 2 ) and high energy-storage efficiency η (92%) were obtained in 2 mol% Pr 3+ -doped PIN-PMN-PT ceramic in the ergodic relaxor (ER) phase at room temperature. The giant electrostrictive effect and excellent energy-storage performance are related to the field-induced dynamic behavior of polar nanoregions (PNRs). The results show that the PIN-PMN-PT:Pr 3+ system is an excellent multifunctional material for making electromechanical and energy storage devices.
研究领域:
材料科学
·
物理学
✓ 已验证
产品关联
DOI
高影响因子
IEEE SENSORS JOURNAL
·
2024
·Vol. 24
·期 16
·26354-26368
·
IF 4.3
Shengwen Shu,Ruojun Yu,Han Qiu,Longlong Shu,Yongling Lu,Zhen Wang
To realize passive vibration monitoring of power transformers, this study proposes a self-powered method for transformer vibration monitoring sensors based on the Sm-doped-Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMN-PT) piezoelectric bimorph array. This study conducts the theoretical analysis and field measurement of the transformer vibration signals. In addition, the preparation method of a high-performance Sm-doped-PMN-PT piezoelectric bimorph is investigated. The properties of the xSm-PMN-yPT ceramics are also analyzed. Further, the output voltage and power characteristics of the piezoelectric bimorph arrays with different combinations are compared. Finally, the validation and application of the prototype are presented. The experimental results show that the 2.5%Sm-PMN-32PT has a high piezoelectric coefficient (d33) of 1710 pC/N. The results also indicate that the piezoelectric self-powered device with a parallel structure consisting of nine piezoelectric bimorphs has a maximum power generation of 2.341 mW under the measured transformer vibration excitation. Moreover, it is shown that it takes 75 min to complete the charging of the 7.5 V-1-F faradic capacitor from 4.4 to 5 V to satisfy the condition for the required energy of 2.82 J for the vibration signal acquisition, processing, and transmission, realizing the intermittent passive vibration monitoring of the transformer for 16 times per day. Therefore, the proposed method has a promising engineering application prospect.
研究领域:
电气工程
·
材料科学
✓ 已验证
DOI
高影响因子
Journal of Advanced Dielectrics
·
2022
·
IF 0
Chuan Chen,Yan Wang,Jiajiu Li,Chaofeng Wu,Guanrong Yang
A series of (100 − x ) Pb(Mg 1 / 3 Nb 2 / 3 ) O 3 − x PbTiO 3 (PMN − x PT, x = 24, 25, 26) ceramics were prepared by solid-state reaction technique using MgNb 2 O 6 precursor. The results of the detailed characterizations reveal that the content of PT has negligible influence on the grain size, and all samples possess the perovskite structure. As the PT content increases, the samples changed from the normal ferroelectric phase to the ergodic relaxor state at room temperature. As a result, PMN– x PT ceramics are endowed with electro-strain of 0.08% at a relatively low electric field of 2 kV/mm, and effective piezoelectric coefficient of 320 pm/V was obtained. Simultaneously, the PMN– x PT ceramics have exceptional pyroelectric performance, exhibiting a high pyroelectric coefficient p ∼ 5.5 – 6.3 × 10 − 8 C⋅cm − 2 ⋅K − 1 . This study demonstrates the great potential of PMN– x PT for piezoelectric and pyroelectric device applications.
研究领域:
材料科学
·
物理学
✓ 已验证
产品关联
DOI
International Journal of Applied Ceramic Technology
·
2024
·Vol. 21
·期 3
·1768-1777
·
IF 1.8
Liang Chen,Changxing Zhao,Peng Jiang,Shuhong Xie,Kai Pan
(1− x )Pb(Mg 1/3 Nb 2/3 )O 3 – x PbTiO 3 (PMN–PT) has attracted attention due to its excellent electrical properties as a typical relaxor ferroelectric material. High-quality Mn–Sm co-doped 0.68PMN–0.32PT thin films were synthesized on the Pt/Ti/SiO 2 /Si substrates by sol–gel based on spin coating method. The results show that 1 mol% Mn–2 mol% Sm co-doped PMN–PT thin films have high dielectric constant ( ε r ∼ 1895) and relatively low dielectric loss (tan δ ∼ .039) at 1 kHz. They also show superior ferroelectric polarization ( P max ∼ 53.71 μC/cm 2 , P r ∼ 30.85 μC/cm 2 ) and high dielectric breakdown strength (∼1656.6 kV/cm), which are primarily due to the low leakage current density (∼10 −7 A/cm 2 ). This work suggests a practical approach to enhance the dielectricity, piezoelectricity, and ferroelectricity of PMN–PT thin films.
研究领域:
材料科学
·
电子工程
✓ 已验证
DOI
高影响因子
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